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@INPROCEEDINGS{Kriehuber:837946,
author = {Kriehuber, Ralf and Dahmen, Volker and Schmitz, Sabine and
Unverricht, Marcus and Pomplun, Ekkehard},
title = {{G}eno- and {C}ytotoxicity of {DNA}-associated {A}uger
{E}lectron emitters},
reportid = {FZJ-2017-06707},
year = {2017},
abstract = {Theoretical considerations, Monte-Carlo simulations and
experimental findings suggest that DNA-incorporated Auger
electron emitters (AEE) cause primarily complex and
clustered DNA lesions. It was previously shown that the
shape of AEE-induced cell survival curves resembles that of
High-LET irradiation and, therefore, poses the question of
an increased biological effectiveness and a separate quality
factor for Auger electrons. During electron capture or
internal conversion an electron vacancy in an inner atomic
shell is created. Filling the electron vacancy by a higher
shell electron can initiate a process of non-radiative
energy transmission, commonly termed as “Auger effect”.
During the process numerous low-energy Auger electrons (up
to 27 in the case of Iodine-125) with a short range are
emitted leading to energy densities and free radical
production in the close vicinity of the emitter exceeding
that of a 5 MeV alpha-particle traversing the DNA
double-helix. Experimental data demonstrate, that the cyto-
and genotoxicity of AEE is comparable to low-LET radiation
per unit dose when the AEE is exclusively located in the
cytoplasm. However, in case of DNA-incorporation RBEs
ranging from 5 – 9 are frequently reported. Employing the
alkaline and neutral comet assay, the high DSB/SSB ratio of
I-125-iododeoxyuridine derived from Monte-Carlo simulations
could be experimentally confirmed. The unique properties of
AEE and the possibility to target DNA in a sequence-specific
manner using AEE-labeled Triplex-forming oligonucleotides
(TFOs) enable to study the repair of complex DNA lesions at
defined sites in more detail. A transgenic SCL-II p2RT
strain carrying the stably integrated recoverable p2RT
vector system harboring a specific triplex target sequence
for TFO-p2RT will help to analyze the repair efficiency of
complex DNA lesions regarding mutation frequency, mutation
type and mutation localization.},
month = {Sep},
date = {2017-09-17},
organization = {Joint Meeting of the European
Radiation Research Society and the
Society for Biological Radiation
Research, Essen (Germany), 17 Sep 2017
- 21 Sep 2017},
subtyp = {After Call},
cin = {S-US},
cid = {I:(DE-Juel1)S-US-20090406},
pnm = {899 - ohne Topic (POF3-899)},
pid = {G:(DE-HGF)POF3-899},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/837946},
}