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@ARTICLE{Staub:838206,
author = {Staub, Florian and Kirchartz, Thomas and Bittkau, Karsten
and Rau, Uwe},
title = {{M}anipulating the {N}et {R}adiative {R}ecombination {R}ate
in {L}ead {H}alide {P}erovskite {F}ilms by {M}odification of
{L}ight {O}utcoupling},
journal = {The journal of physical chemistry letters},
volume = {8},
issn = {1948-7185},
address = {Washington, DC},
publisher = {ACS},
reportid = {FZJ-2017-06868},
pages = {5084 - 5090},
year = {2017},
abstract = {Photon recycling is a fundamental physical process that
becomes especially important for photovoltaic devices that
operate close to the radiative limit. This implies that the
externally measured radiative decay rate deviates from the
internal radiative recombination rate of the material. In
the present Letter, the probability of photon recycling in
organic lead halide perovskite films is manipulated by
modifying the underlying layer stacks. We observe
recombination kinetics by time-resolved photoluminescence
that is controlled by the optical design of the chosen layer
structure. Quantitative simulations of decay rates and
emission spectra show excellent agreement with experimental
results if we assume that the internal bimolecular
recombination coefficient is ~ 66 $\%$ radiative.},
cin = {IEK-5},
ddc = {530},
cid = {I:(DE-Juel1)IEK-5-20101013},
pnm = {121 - Solar cells of the next generation (POF3-121) / HITEC
- Helmholtz Interdisciplinary Doctoral Training in Energy
and Climate Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF3-121 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:28976758},
UT = {WOS:000413798300019},
doi = {10.1021/acs.jpclett.7b02224},
url = {https://juser.fz-juelich.de/record/838206},
}