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000838452 1001_ $$0P:(DE-Juel1)130389$$aNeumeier, Stefan$$b0$$eCorresponding author
000838452 245__ $$aNew insights into phosphate based materials for the immobilisation of actinides
000838452 260__ $$aBerlin$$bDe Gruyter$$c2017
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000838452 520__ $$aThis paper focuses on major phosphate-based ceramic materials relevant for the immobilisation of Pu, minor actinides, fission and activation products. Key points addressed include the recent progress regarding synthesis methods, the formation of solid solutions by structural incorporation of actinides or their non-radioactive surrogates and waste form fabrication by advanced sintering techniques. Particular attention is paid to the properties that govern the long-term stability of the waste forms under conditions relevant to geological disposal. The paper highlights the benefits gained from synergies of state-of-the-art experimental approaches and advanced atomistic modeling tools for addressing properties and stability of f-element-bearing phosphate materials. In conclusion, this article provides a perspective on the recent advancements in the understanding of phosphate based ceramics and their properties with respect to their application as nuclear waste forms.
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000838452 7001_ $$0P:(DE-Juel1)171900$$aArinicheva, Yulia$$b1
000838452 7001_ $$0P:(DE-Juel1)137024$$aKowalski, Piotr$$b2
000838452 7001_ $$0P:(DE-Juel1)159378$$aKegler, Philip$$b3
000838452 7001_ $$0P:(DE-Juel1)133034$$aSchlenz, Hartmut$$b4
000838452 7001_ $$0P:(DE-Juel1)130324$$aBosbach, Dirk$$b5
000838452 7001_ $$0P:(DE-Juel1)156511$$aDeissmann, Guido$$b6
000838452 7001_ $$0P:(DE-Juel1)142369$$aHeuser, Julia$$b7
000838452 7001_ $$0P:(DE-Juel1)165842$$aJi, Yaqi$$b8$$ufzj
000838452 773__ $$0PERI:(DE-600)2039575-9$$a10.1515/ract-2017-2819$$gVol. 0, no. 0$$n11$$p961-984$$tRadiochimica acta$$v105$$x2193-3405$$y2017
000838452 8564_ $$uhttps://juser.fz-juelich.de/record/838452/files/%5BRadiochimica%20Acta%5D%20New%20insights%20into%20phosphate%20based%20materials%20for%20the%20immobilisation%20of%20actinides.pdf$$yPublished on 2017-10-12. Available in OpenAccess from 2018-10-12.
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000838452 8564_ $$uhttps://juser.fz-juelich.de/record/838452/files/%5BRadiochimica%20Acta%5D%20New%20insights%20into%20phosphate%20based%20materials%20for%20the%20immobilisation%20of%20actinides.jpg?subformat=icon-180$$xicon-180$$yPublished on 2017-10-12. Available in OpenAccess from 2018-10-12.
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