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@ARTICLE{Neumeier:838452,
author = {Neumeier, Stefan and Arinicheva, Yulia and Kowalski, Piotr
and Kegler, Philip and Schlenz, Hartmut and Bosbach, Dirk
and Deissmann, Guido and Heuser, Julia and Ji, Yaqi},
title = {{N}ew insights into phosphate based materials for the
immobilisation of actinides},
journal = {Radiochimica acta},
volume = {105},
number = {11},
issn = {2193-3405},
address = {Berlin},
publisher = {De Gruyter},
reportid = {FZJ-2017-07055},
pages = {961-984},
year = {2017},
abstract = {This paper focuses on major phosphate-based ceramic
materials relevant for the immobilisation of Pu, minor
actinides, fission and activation products. Key points
addressed include the recent progress regarding synthesis
methods, the formation of solid solutions by structural
incorporation of actinides or their non-radioactive
surrogates and waste form fabrication by advanced sintering
techniques. Particular attention is paid to the properties
that govern the long-term stability of the waste forms under
conditions relevant to geological disposal. The paper
highlights the benefits gained from synergies of
state-of-the-art experimental approaches and advanced
atomistic modeling tools for addressing properties and
stability of f-element-bearing phosphate materials. In
conclusion, this article provides a perspective on the
recent advancements in the understanding of phosphate based
ceramics and their properties with respect to their
application as nuclear waste forms.},
cin = {IEK-6 / IEK-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-6-20101013 / I:(DE-Juel1)IEK-1-20101013},
pnm = {161 - Nuclear Waste Management (POF3-161) / HITEC -
Helmholtz Interdisciplinary Doctoral Training in Energy and
Climate Research (HITEC) (HITEC-20170406)},
pid = {G:(DE-HGF)POF3-161 / G:(DE-Juel1)HITEC-20170406},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000415589500006},
doi = {10.1515/ract-2017-2819},
url = {https://juser.fz-juelich.de/record/838452},
}