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@INPROCEEDINGS{Freimuth:838610,
author = {Freimuth, Frank},
title = {{L}aser excitation of photocurrents in inversion asymmetric
ferromagnets},
reportid = {FZJ-2017-07187},
year = {2017},
abstract = {By breaking the inversion symmetry in crystals one enables
several mechanisms for photocurrent generation, which
otherwise would be forbidden by symmetry. First, there is
the circular photogalvanic effect [1,2], which has recently
attracted attention in noncentrosymmetric Weyl semimetals
[3,4]. Since most previous works on the circular
photogalvanic effect have focused on nonmagnetic
semiconductors, in this talk we will discuss this effect in
ferromagnetic metals. Second, when magnetic solids are
excited by femtosecond laser pulses, superdiffusive spin
currents are generated, which are converted into charge
currents by the inverse spin Hall effect [5,6]. Third,
photocurrents are also generated when magnetization dynamics
is excited by laser pulses, because magnetization dynamics
pumps electrical currents due to the inverse spin‐orbit
torque (ISOT) [7]. At small frequencies, i.e., under typical
FMR conditions, the inverse spin‐orbit torque can be
understood in terms of spin pumping combined with the spin
Hall effect and in terms of the Rashba or Dresselhaus
spin‐orbit fields [8,9,10,11]. However, when magnetic
solids are excited by femtosecond laser pulses, additional
effects set in, such as ultrafast demagnetization, which
lead to new mechanisms for generating electrical currents in
inversion asymmetric magnets. These photocurrents provide a
new tool to probe magnetization dynamics at subpicosecond
time scales. Using the Keldysh formalism we systematically
identify mechanisms behind the generation of electrical
currents in the range from FMR up to optical frequencies,
discovering also several new effects. In particular, we find
that not only precession of magnetization, but also
demagnetization, drives photocurrents [12]. Based on DFT
calculations we investigate these effects in Co/Pt and Mn/W
bilayers and elucidate the role that spin‐currents play.
The inverse Faraday effect (IFE) and the optical
spin‐transfer torque (OSTT) can be used to excite
magnetization dynamics by femtosecond laser pulses. We
present ab‐initio calculations of IFE and OSTT in Fe, Co
and FePt, compare the relative magnitude of IFE and OSTT in
these materials and discuss the disorder dependence[13].[1]
J. W. McIver et al., Nature Nanotechnology 7, 96 (2012) [2]
S. D. Ganichev and W. Prettl, JPCM 15, R935 (2003) [3] H.
Ishizuka et al., PRL 117, 216601 (2016) [4] Q. Ma et al.,
Nature Physics, DOI:10.1038/NPHYS4146 (2017) [5] T.
Kampfrath et al., Nature Nanotechnology 8, 256 (2013) [6] T.
Seifert et al., Nature Photonics 10, 483 (2016) [7] T. J.
Huisman et al., Nature Nanotechnology 11, 455 (2016)[8] F.
Freimuth, S. Blügel and Y. Mokrousov, PRB 90, 174423
(2014) [9] F. Freimuth, S. Blügel and Y. Mokrousov, JPCM
26, 104202 (2014) [10] F. Freimuth, S. Blügel and Y.
Mokrousov, PRB 92, 064415 (2015) [11] F. Freimuth, S.
Blügel and Y. Mokrousov, JPCM 28, 316001 (2016) [12] F.
Freimuth, S. Blügel and Y. Mokrousov, PRB 95, 094434
(2017) [13] F. Freimuth, S. Blügel and Y. Mokrousov, PRB
94, 144432 (2016)},
month = {Oct},
date = {2017-10-09},
organization = {Ultrafast Magnetism Conference,
Kaiserslautern (Germany), 9 Oct 2017 -
13 Oct 2017},
subtyp = {Other},
cin = {IAS-1 / PGI-1 / JARA-FIT / JARA-HPC},
cid = {I:(DE-Juel1)IAS-1-20090406 / I:(DE-Juel1)PGI-1-20110106 /
$I:(DE-82)080009_20140620$ / $I:(DE-82)080012_20140620$},
pnm = {142 - Controlling Spin-Based Phenomena (POF3-142)},
pid = {G:(DE-HGF)POF3-142},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/838610},
}