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@ARTICLE{Jurkat:838639,
author = {Jurkat, T. and Voigt, C. and Kaufmann, S. and Grooß, J.-U.
and Ziereis, H. and Dörnbrack, A. and Hoor, P. and Bozem,
H. and Engel, A. and Bönisch, H. and Keber, T. and Hüneke,
T. and Pfeilsticker, K. and Zahn, A. and Walker, K. A. and
Boone, C. D. and Bernath, P. F. and Schlager, H.},
title = {{D}epletion of ozone and reservoir species of chlorine and
nitrogen oxide in the lower {A}ntarctic polar vortex
measured from aircraft},
journal = {Geophysical research letters},
volume = {44},
number = {12},
issn = {0094-8276},
address = {Hoboken, NJ},
publisher = {Wiley},
reportid = {FZJ-2017-07212},
pages = {6440 - 6449},
year = {2017},
abstract = {Novel airborne in situ measurements of inorganic chlorine,
nitrogen oxide species, and ozone were performed inside the
lower Antarctic polar vortex and at its edge in September
2012. We focus on one flight during the Transport and
Composition of the LMS/Earth System Model Validation
(TACTS/ESMVal) campaign with the German research aircraft
HALO (High-Altitude LOng range research aircraft), reaching
latitudes of 65°S and potential temperatures up to 405 K.
Using the early winter correlations of reactive trace gases
with N2O from the Atmospheric Chemistry Experiment-Fourier
Transform Spectrometer (ACE-FTS), we find high depletion of
chlorine reservoir gases up to $∼40\%$ (0.8 ppbv) at 12 km
to 14 km altitude in the vortex and 0.4 ppbv at the edge in
subsided stratospheric air with mean ages up to 4.5 years.
We observe denitrification of up to 4 ppbv, while ozone was
depleted by 1.2 ppmv at potential temperatures as low as 380
K. The advanced instrumentation aboard HALO enables
high-resolution measurements with implications for the
oxidation capacity of the lowermost stratosphere.},
cin = {IEK-7},
ddc = {550},
cid = {I:(DE-Juel1)IEK-7-20101013},
pnm = {244 - Composition and dynamics of the upper troposphere and
middle atmosphere (POF3-244)},
pid = {G:(DE-HGF)POF3-244},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000405854200065},
doi = {10.1002/2017GL073270},
url = {https://juser.fz-juelich.de/record/838639},
}