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000838700 1001_ $$0P:(DE-HGF)0$$aHunter, James F.$$b0
000838700 245__ $$aComprehensive characterization of atmospheric organic carbon at a forested site
000838700 260__ $$aLondon$$bNature Publ. Group$$c2017
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000838700 520__ $$aAtmospheric organic compounds are central to key chemical processes that influence air quality, ecological health, and climate. However, longstanding difficulties in predicting important quantities such as organic aerosol formation and oxidant lifetimes indicate that our understanding of atmospheric organic chemistry is fundamentally incomplete, probably due in part to the presence of organic species that are unmeasured using standard analytical techniques. Here we present measurements of a wide range of atmospheric organic compounds—including previously unmeasured species—taken concurrently at a single site (a ponderosa pine forest during summertime) by five state-of-the-art mass spectrometric instruments. The combined data set provides a comprehensive characterization of atmospheric organic carbon, covering a wide range in chemical properties (volatility, oxidation state, and molecular size), and exhibiting no obvious measurement gaps. This enables the first construction of a measurement-based local organic budget, highlighting the high emission, deposition, and oxidation fluxes in this environment. Moreover, previously unmeasured species, including semivolatile and intermediate-volatility organic species (S/IVOCs), account for one-third of the total organic carbon, and (within error) provide closure on both OH reactivity and potential secondary organic aerosol formation.
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000838700 7001_ $$0P:(DE-HGF)0$$aDay, Douglas A.$$b1
000838700 7001_ $$0P:(DE-HGF)0$$aPalm, Brett B.$$b2
000838700 7001_ $$0P:(DE-HGF)0$$aYatavelli, Reddy L. N.$$b3
000838700 7001_ $$0P:(DE-HGF)0$$aChan, Arthur W. H.$$b4
000838700 7001_ $$0P:(DE-HGF)0$$aKaser, Lisa$$b5
000838700 7001_ $$0P:(DE-HGF)0$$aCappellin, Luca$$b6
000838700 7001_ $$0P:(DE-HGF)0$$aHayes, Patrick L.$$b7
000838700 7001_ $$0P:(DE-HGF)0$$aCross, Eben S.$$b8
000838700 7001_ $$0P:(DE-HGF)0$$aCarrasquillo, Anthony J.$$b9
000838700 7001_ $$0P:(DE-HGF)0$$aCampuzano-Jost, Pedro$$b10
000838700 7001_ $$0P:(DE-HGF)0$$aStark, Harald$$b11
000838700 7001_ $$0P:(DE-HGF)0$$aZhao, Yunliang$$b12
000838700 7001_ $$0P:(DE-Juel1)161442$$aHohaus, Thorsten$$b13$$ufzj
000838700 7001_ $$0P:(DE-HGF)0$$aSmith, James N.$$b14
000838700 7001_ $$0P:(DE-HGF)0$$aHansel, Armin$$b15
000838700 7001_ $$0P:(DE-HGF)0$$aKarl, Thomas$$b16
000838700 7001_ $$0P:(DE-HGF)0$$aGoldstein, Allen H.$$b17
000838700 7001_ $$0P:(DE-HGF)0$$aGuenther, Alex$$b18
000838700 7001_ $$0P:(DE-HGF)0$$aWorsnop, Douglas R.$$b19
000838700 7001_ $$0P:(DE-HGF)0$$aThornton, Joel A.$$b20
000838700 7001_ $$0P:(DE-HGF)0$$aHeald, Colette L.$$b21
000838700 7001_ $$0P:(DE-HGF)0$$aJimenez, Jose L.$$b22
000838700 7001_ $$0P:(DE-HGF)0$$aKroll, Jesse H.$$b23$$eCorresponding author
000838700 773__ $$0PERI:(DE-600)2396648-8$$a10.1038/ngeo3018$$gVol. 10, no. 10, p. 748 - 753$$n10$$p748 - 753$$tNature geoscience$$v10$$x1752-0908$$y2017
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