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@ARTICLE{Hunter:838700,
      author       = {Hunter, James F. and Day, Douglas A. and Palm, Brett B. and
                      Yatavelli, Reddy L. N. and Chan, Arthur W. H. and Kaser,
                      Lisa and Cappellin, Luca and Hayes, Patrick L. and Cross,
                      Eben S. and Carrasquillo, Anthony J. and Campuzano-Jost,
                      Pedro and Stark, Harald and Zhao, Yunliang and Hohaus,
                      Thorsten and Smith, James N. and Hansel, Armin and Karl,
                      Thomas and Goldstein, Allen H. and Guenther, Alex and
                      Worsnop, Douglas R. and Thornton, Joel A. and Heald,
                      Colette L. and Jimenez, Jose L. and Kroll, Jesse H.},
      title        = {{C}omprehensive characterization of atmospheric organic
                      carbon at a forested site},
      journal      = {Nature geoscience},
      volume       = {10},
      number       = {10},
      issn         = {1752-0908},
      address      = {London},
      publisher    = {Nature Publ. Group},
      reportid     = {FZJ-2017-07262},
      pages        = {748 - 753},
      year         = {2017},
      abstract     = {Atmospheric organic compounds are central to key chemical
                      processes that influence air quality, ecological health, and
                      climate. However, longstanding difficulties in predicting
                      important quantities such as organic aerosol formation and
                      oxidant lifetimes indicate that our understanding of
                      atmospheric organic chemistry is fundamentally incomplete,
                      probably due in part to the presence of organic species that
                      are unmeasured using standard analytical techniques. Here we
                      present measurements of a wide range of atmospheric organic
                      compounds—including previously unmeasured species—taken
                      concurrently at a single site (a ponderosa pine forest
                      during summertime) by five state-of-the-art mass
                      spectrometric instruments. The combined data set provides a
                      comprehensive characterization of atmospheric organic
                      carbon, covering a wide range in chemical properties
                      (volatility, oxidation state, and molecular size), and
                      exhibiting no obvious measurement gaps. This enables the
                      first construction of a measurement-based local organic
                      budget, highlighting the high emission, deposition, and
                      oxidation fluxes in this environment. Moreover, previously
                      unmeasured species, including semivolatile and
                      intermediate-volatility organic species (S/IVOCs), account
                      for one-third of the total organic carbon, and (within
                      error) provide closure on both OH reactivity and potential
                      secondary organic aerosol formation.},
      cin          = {IEK-8},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000412102200011},
      doi          = {10.1038/ngeo3018},
      url          = {https://juser.fz-juelich.de/record/838700},
}