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@ARTICLE{CabreraPerez:838785,
      author       = {Cabrera-Perez, David and Taraborrelli, Domenico and
                      Lelieveld, Jos and Hoffmann, Thorsten and Pozzer, Andrea},
      title        = {{G}lobal impact of monocyclic aromatics on tropospheric
                      composition},
      journal      = {Atmospheric chemistry and physics / Discussions},
      volume       = {928},
      issn         = {1680-7375},
      address      = {Katlenburg-Lindau},
      publisher    = {EGU},
      reportid     = {FZJ-2017-07310},
      pages        = {1 - 25},
      year         = {2017},
      abstract     = {Aromatic compounds are reactive species influencing ozone
                      formation, OH concentrations and organic aerosol formation.
                      An assessment of their impacts on the gas-phase composition
                      at a global scale has been performed using a general
                      circulation atmospheric-chemistry model.Globally, we found a
                      small annual average net decrease (less than $3 \%)$ in
                      global OH, ozone, and NOx mixing ratios when aromatic
                      compounds are included in the chemical mechanism. This
                      inclusion of aromatics also results in CO mixing ratio
                      increases, which cause a general decrease in OH
                      concentrations. The largest changes are found in glyoxal and
                      NO3, with increases in the atmospheric burden of $10 \%$
                      and $6 \%,$ respectively.Regionally, significant
                      differences were found particularly in high NOx regime
                      areas, with an increase of up to $4 \%$ in O3 mixing
                      ratios and $8 \%$ in OH concentrations. NO3 increased by
                      more than $30 \%$ in several regions of the northern
                      hemisphere, and glyoxal increased up to $40 \%$ in Europe
                      and Asia. Large increases in formaldehyde were found in
                      urban areas.Although the relative impact of aromatics at the
                      global scale is limited, at a regional level they are
                      important in atmospheric chemistry.},
      cin          = {IEK-8},
      ddc          = {550},
      cid          = {I:(DE-Juel1)IEK-8-20101013},
      pnm          = {243 - Tropospheric trace substances and their
                      transformation processes (POF3-243)},
      pid          = {G:(DE-HGF)POF3-243},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.5194/acp-2017-928},
      url          = {https://juser.fz-juelich.de/record/838785},
}