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@ARTICLE{Niebuur:838859,
      author       = {Niebuur, Bart-Jan and Claude, Kora-Lee and Pinzek, Simon
                      and Cariker, Coleman and Raftopoulos, Konstantinos N. and
                      Pipich, Vitaliy and Appavou, Marie-Sousai and Schulte,
                      Alfons and Papadakis, Christine M.},
      title        = {{P}ressure-{D}ependence of {P}oly( {N}
                      -isopropylacrylamide) {M}esoglobule {F}ormation in {A}queous
                      {S}olution},
      journal      = {ACS Macro Letters},
      volume       = {6},
      number       = {11},
      issn         = {2161-1653},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2017-07369},
      pages        = {1180 - 1185},
      year         = {2017},
      abstract     = {Above their cloud point, aqueous solutions of the
                      thermoresponsive polymer poly(N-isopropylacrylamide)
                      (PNIPAM) form large mesoglobules. We have carried out very
                      small-angle neutron scattering (VSANS with q = 0.21–2.3 ×
                      10–3 Å–1) and Raman spectroscopy experiments on a 3 wt
                      $\%$ PNIPAM solution in D2O at atmospheric and elevated
                      pressures (up to 113 MPa). Raman spectroscopy reveals that,
                      at high pressure, the polymer is less dehydrated upon
                      crossing the cloud point. VSANS shows that the mesoglobules
                      are significantly larger and contain more D2O than at
                      atmospheric pressure. We conclude that the size of the
                      mesoglobules and thus their growth process are closely
                      related to the hydration state of PNIPAM.},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
                      6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)},
      pid          = {G:(DE-HGF)POF3-6215 / G:(DE-HGF)POF3-6G4},
      experiment   = {EXP:(DE-MLZ)KWS3-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000416500000001},
      doi          = {10.1021/acsmacrolett.7b00563},
      url          = {https://juser.fz-juelich.de/record/838859},
}