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@ARTICLE{BarEyal:838861,
author = {Bar Eyal, Leeat and Ranjbar Choubeh, Reza and Cohen, Eyal
and Eisenberg, Ido and Tamburu, Carmen and Dorogi, Márta
and Ünnep, Renata and Appavou, Marie-Sousai and Nevo,
Reinat and Raviv, Uri and Reich, Ziv and Garab, Győző and
van Amerongen, Herbert and Paltiel, Yossi and Keren, Nir},
title = {{C}hanges in aggregation states of light-harvesting
complexes as a mechanism for modulating energy transfer in
desert crust cyanobacteria},
journal = {Proceedings of the National Academy of Sciences of the
United States of America},
volume = {114},
number = {35},
issn = {1091-6490},
address = {Washington, DC},
publisher = {National Acad. of Sciences},
reportid = {FZJ-2017-07371},
pages = {9481 - 9486},
year = {2017},
abstract = {In this paper we propose an energy dissipation mechanism
that is completely reliant on changes in the aggregation
state of the phycobilisome light-harvesting antenna
components. All photosynthetic organisms regulate the
efficiency of excitation energy transfer (EET) to fit light
energy supply to biochemical demands. Not many do this to
the extent required of desert crust cyanobacteria. Following
predawn dew deposition, they harvest light energy with
maximum efficiency until desiccating in the early morning
hours. In the desiccated state, absorbed energy is
completely quenched. Time and spectrally resolved
fluorescence emission measurements of the desiccated desert
crust Leptolyngbya ohadii strain identified (i) reduced EET
between phycobilisome components, (ii) shorter fluorescence
lifetimes, and (iii) red shift in the emission spectra,
compared with the hydrated state. These changes coincide
with a loss of the ordered phycobilisome structure, evident
from small-angle neutron and X-ray scattering and
cryo-transmission electron microscopy data. Based on these
observations we propose a model where in the hydrated state
the organized rod structure of the phycobilisome supports
directional EET to reaction centers with minimal losses due
to thermal dissipation. In the desiccated state this
structure is lost, giving way to more random aggregates. The
resulting EET path will exhibit increased coupling to the
environment and enhanced quenching.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {000},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)KWS2-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:28808031},
UT = {WOS:000408536000067},
doi = {10.1073/pnas.1708206114},
url = {https://juser.fz-juelich.de/record/838861},
}