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@ARTICLE{Weber:839914,
author = {Weber, T. and Roessli, B. and Stock, C. and Keller, T. and
Schmalzl, K. and Bourdarot, F. and Georgii, R. and Ewings,
R. A. and Perry, R. S. and Böni, P.},
title = {{T}ransverse acoustic phonon anomalies at intermediate wave
vectors in {M}g{V} 2 {O} 4},
journal = {Physical review / B},
volume = {96},
number = {18},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2017-07492},
pages = {184301},
year = {2017},
abstract = {Magnetic spinels (with chemical formula AX2O4, with X a 3d
transition metal ion) that also have an orbital degeneracy
are Jahn-Teller active and hence possess a coupling between
spin and lattice degrees of freedom. At high temperatures,
MgV2O4 is a cubic spinel based on V3+ ions with a spin S=1
and a triply degenerate orbital ground state. A structural
transition occurs at TOO=63 K to an orbitally ordered phase
with a tetragonal unit cell followed by an antiferromagnetic
transition of TN=42 K on cooling. We apply neutron
spectroscopy in single crystals of MgV2O4 to show an anomaly
for intermediate wave vectors at TOO associated with the
acoustic phonon sensitive to the shear elastic modulus
(C11−C12)/2. On warming, the shear mode softens for
momentum transfers near close to half the Brillouin zone
boundary, but recovers near the zone center. High resolution
spin-echo measurements further illustrate a temporal
broadening with increased temperature over this intermediate
range of wave vectors, indicative of a reduction in phonon
lifetime. A subtle shift in phonon frequencies over the same
range of momentum transfers is observed with magnetic
fields. We discuss this acoustic anomaly in context of
coupling to orbital and charge fluctuations.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS-ILL},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ / I:(DE-Juel1)JCNS-ILL-20110128},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-Juel1)ILL-IN12-20150421},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000414526200004},
doi = {10.1103/PhysRevB.96.184301},
url = {https://juser.fz-juelich.de/record/839914},
}