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@ARTICLE{Buchold:839924,
author = {Buchold, Philipp and Schweins, Ralf and Di, Zhenyu and
Gradzielski, Michael},
title = {{S}tructural behaviour of sodium hyaluronate in
concentrated oppositely charged surfactant solutions},
journal = {Soft matter},
volume = {13},
number = {11},
issn = {1744-6848},
address = {London},
publisher = {Royal Soc. of Chemistry},
reportid = {FZJ-2017-07502},
pages = {2253 - 2263},
year = {2017},
abstract = {This work discusses the polyelectrolyte sodium hyaluronate
(HA) and its polyelectrolyte/surfactant complexes (PESCs)
with tetradecyltrimethylammonium bromide (TTAB) in the
semi-dilute regime of HA and at high concentrations of TTAB.
The structure and flow properties in the surfactant excess
region were studied by light scattering and small angle
neutron scattering (SANS) as well as by rheology. The unique
behaviour of HA to maintain its high viscosity was observed
even at very high TTAB concentrations of 496 mM and this
effect was systematically studied in the concentration range
from 1 to 25 mM HA. From the data, it could be concluded
that: (1) extended rod-like structures of the PESCs prevent
molecular dissolution of HA by TTAB. (2) HA and TTAB
micelles interact rather weakly as seen by a low fraction of
bound micelles. (3) At very high TTAB concentrations a
decompaction of PESCs (fractal dimension Df going from 2.0
to 1.2) occurs with increasing HA concentration but (4) both
the entanglement of HA and the structure of the micelles are
not affected.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6G15 - FRM II / MLZ (POF3-6G15)},
pid = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
experiment = {EXP:(DE-MLZ)KWS2-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:28261739},
UT = {WOS:000397955800014},
doi = {10.1039/C6SM02742C},
url = {https://juser.fz-juelich.de/record/839924},
}