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@ARTICLE{Papadakis:839929,
      author       = {Papadakis, Christine and Tsitsilianis, Constantinos},
      title        = {{R}esponsive {H}ydrogels from {A}ssociative {B}lock
                      {C}opolymers: {P}hysical {G}elling through {P}olyion
                      {C}omplexation},
      journal      = {Gels},
      volume       = {3},
      number       = {1},
      issn         = {2310-2861},
      address      = {Basel},
      publisher    = {MDPI},
      reportid     = {FZJ-2017-07507},
      pages        = {3 -},
      year         = {2017},
      abstract     = {The present review article highlights a specific class of
                      responsive polymer-based hydrogels which are formed through
                      association of oppositely charged polyion segments. The
                      underpinning temporary three-dimensional network is
                      constituted of hydrophilic chains (either ionic or neutral)
                      physically crosslinked by ion pair formation arising from
                      intermolecular polyionic complexation of oppositely charged
                      repeating units (polyacid/polybase ionic interactions). Two
                      types of hydrogels are presented: (i) hydrogels formed by
                      triblock copolymers bearing oppositely charged blocks (block
                      copolyampholytes), forming self-assembled networks; and (ii)
                      hydrogels formed by co-assembly of oppositely charged
                      polyelectrolyte segments belonging to different
                      macromolecules (either block copolymers or
                      homopolyelectrolytes). Due to the weak nature of the
                      involved polyions, these hydrogels respond to pH and are
                      sensitive to the presence of salts. Discussing and
                      evaluating their solution, rheological and structural
                      properties in dependence on pH and ionic strength, it comes
                      out that the hydrogel properties are tunable towards
                      potential applications},
      cin          = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
                      (München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
                      / 6G15 - FRM II / MLZ (POF3-6G15)},
      pid          = {G:(DE-HGF)POF3-6G4 / G:(DE-HGF)POF3-6G15},
      experiment   = {EXP:(DE-MLZ)KWS2-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:30920500},
      UT           = {WOS:000461121500003},
      doi          = {10.3390/gels3010003},
      url          = {https://juser.fz-juelich.de/record/839929},
}