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@ARTICLE{Uhlenbruck:840019,
author = {Uhlenbruck, Sven and Dornseiffer, Jürgen and Lobe, Sandra
and Dellen, Christian and Tsai, Chih-Long and Gotzen,
Benjamin and Sebold, Doris and Finsterbusch, Martin and
Guillon, Olivier},
title = {{C}athode-electrolyte material interactions during
manufacturing of inorganic solid-state lithium batteries},
journal = {Journal of electroceramics},
volume = {38},
number = {2-4},
issn = {1385-3449},
address = {Dordrecht [u.a.]},
publisher = {Springer Science + Business Media B.V},
reportid = {FZJ-2017-07589},
pages = {197 - 206},
year = {2017},
abstract = {Solid-state lithium batteries comprising a ceramic
electrolyte instead of a liquid one enable safer high-energy
batteries. Their manufacturing usually requires a high
temperature heat treatment to interconnect electrolyte,
electrodes, and if applicable, further components like
current collectors. Tantalum-substituted Li7La3Zr2O12 as
electrolyte and LiCoO2 as active material on the cathode
side were chosen because of their high ionic conductivity
and energy density, respectively. However, both materials
react severely with each other at temperatures around 1085
°C thus leading to detrimental secondary phases. Thin-film
technologies open a pathway for manufacturing compounds of
electrolyte and active material at lower processing
temperatures. Two of them are addressed in this work to
manufacture thin electrolyte layers of the aforementioned
materials at low temperatures: physical vapor deposition and
coating technologies with liquid precursors. They are
especially applicable for electrolyte layers since
electrolytes require a high density while at the same time
their thickness can be as thin as possible, provided that
the separation of the electrodes is still guaranteed.},
cin = {IEK-1},
ddc = {620},
cid = {I:(DE-Juel1)IEK-1-20101013},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000415362700009},
doi = {10.1007/s10832-016-0062-x},
url = {https://juser.fz-juelich.de/record/840019},
}