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@ARTICLE{Murmann:840039,
author = {Murmann, Patrick and Börner, Markus and Cekic-Laskovic,
Isidora and Winter, Martin},
title = {{I}nfluence of
lithium-cyclo-difluoromethane-1,1-bis(sulfonyl)imide as
electrolyte additive on the reversibility of lithium metal
batteries},
journal = {Journal of applied electrochemistry},
volume = {46},
number = {3},
issn = {1572-8838},
address = {Dordrecht [u.a.]},
publisher = {Springer Science + Business Media B.V},
reportid = {FZJ-2017-07605},
pages = {339 - 348},
year = {2016},
abstract = {Electrolyte solutions containing
lithium-cyclo-difluoromethane-1,1-bis(sulfonyl)imide
(LiDMSI) as an additive were specifically designed for
measurements in lithium plating-stripping model experiments
on copper electrodes. LiDMSI was implemented into two
different electrolyte solutions. The first electrolyte setup
consisted of a 1 M solution of LiTFSI in PC as an
electrolyte which is known to show a comparably limited
performance for reversible Li deposition. The second setup
was comprised 1 M LiAsF6 in 1,3-dioxolane as the base
electrolyte which depicts a well-tested performance for
lithium deposition–dissolution. The addition of LiDMSI
yielded significantly improved results in regard to
Coulombic efficiencies and cycling stability in both
electrolyte compositions. Furthermore, it negated the
formation of high surface area, e.g., dendritic lithium,
which depicts the main source for the limited safety of
rechargeable lithium metal batteries. In the case of the
PC-based electrolyte system, the LiDMSI-containing
electrolyte illustrates a slightly lowered over-potential on
the copper substrate, while for the dioxolane-based setup
the over-potentials were almost completely equal. In order
to compare the morphologies of the lithium deposits, SEM
images were utilized.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000371469400008},
doi = {10.1007/s10800-016-0924-6},
url = {https://juser.fz-juelich.de/record/840039},
}