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@ARTICLE{Murmann:840040,
author = {Murmann, Patrick and Mönnighoff, Xaver and von Aspern,
Natascha and Janssen, Pia and Kalinovich, Nataliya and
Shevchuk, Michael and Kazakova, Olesya and Röschenthaler,
Gerd-Volker and Cekic-Laskovic, Isidora and Winter, Martin},
title = {{I}nfluence of the {F}luorination {D}egree of
{O}rganophosphates on {F}lammability and {E}lectrochemical
{P}erformance in {L}ithium {I}on {B}atteries: {S}tudies on
{F}luorinated {C}ompounds {D}eriving from {T}riethyl
{P}hosphate},
journal = {Journal of the Electrochemical Society},
volume = {163},
number = {5},
issn = {1945-7111},
address = {Pennington, NJ},
publisher = {Electrochemical Soc.},
reportid = {FZJ-2017-07606},
pages = {A751 - A757},
year = {2016},
abstract = {Three symmetric substances originating from triethyl
phosphate were specifically synthesized with varying degree
of fluorination at the side chain. Different concentrations
of each phosphate were evaluated as co-solvent with regard
to their flammability and the electrochemical cycling
performance. With higher degree of fluorination and a higher
amount of the phosphate in the electrolyte, the
self-extinguishing time (SET), a value to determine and
compare the flammability of electrolytes, could be
significantly lowered to yield a non-flammable electrolyte
mixture. A specifically designed SET device is introduced,
which offers more accurate results due to lowered standard
deviations by minimizing random and systematic errors. As
the application of phosphates as co-solvents results in a
trade-off in cycling performance, a thorough determination
in regard to the ionic conductivity, the anodic oxidation
stability and the compatibility with anode and cathode
material was carried out in half- and full-cells. The
manuscript strives to establish a deeper understanding of
the influence that the utilization of phosphates as
co-solvents entail with special focus on the fluorination
degree. It could be shown that the partially fluorinated
phosphate offers the best cycling results and therefore the
lowest trade-off in performance, while a severe improvement
in SET could be achieved compared to the reference
electrolyte.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {131 - Electrochemical Storage (POF3-131)},
pid = {G:(DE-HGF)POF3-131},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000370866700023},
doi = {10.1149/2.1031605jes},
url = {https://juser.fz-juelich.de/record/840040},
}