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000840068 1001_ $$0P:(DE-Juel1)156558$$aGottselig, N.$$b0
000840068 245__ $$aElemental Composition of Natural Nanoparticles and Fine Colloids in European Forest Stream Waters and Their Role as Phosphorus Carriers
000840068 260__ $$aHoboken, NJ$$bWiley$$c2017
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000840068 520__ $$aBiogeochemical cycling of elements largely occurs in dissolved state, but many elements may also be bound to natural nanoparticles (NNP, 1–100 nm) and fine colloids (100–450 nm). We examined the hypothesis that the size and composition of stream water NNP and colloids vary systematically across Europe. To test this hypothesis, 96 stream water samples were simultaneously collected in 26 forested headwater catchments along two transects across Europe. Three size fractions (~1–20 nm, >20–60 nm, and >60 nm) of NNP and fine colloids were identified with Field Flow Fractionation coupled to inductively coupled plasma mass spectrometry and an organic carbon detector. The results showed that NNP and fine colloids constituted between 2 ± 5% (Si) and 53 ± 21% (Fe; mean ± SD) of total element concentrations, indicating a substantial contribution of particles to element transport in these European streams, especially for P and Fe. The particulate contents of Fe, Al, and organic C were correlated to their total element concentrations, but those of particulate Si, Mn, P, and Ca were not. The fine colloidal fractions >60 nm were dominated by clay minerals across all sites. The resulting element patterns of NNP <60 nm changed from North to South Europe from Fe- to Ca-dominated particles, along with associated changes in acidity, forest type, and dominant lithology.
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000840068 7001_ $$0P:(DE-Juel1)129427$$aAmelung, Wulf$$b1
000840068 7001_ $$00000-0001-6577-3619$$aKirchner, J. W.$$b2
000840068 7001_ $$0P:(DE-Juel1)145865$$aBol, R.$$b3
000840068 7001_ $$00000-0001-6067-0741$$aEugster, W.$$b4
000840068 7001_ $$0P:(DE-HGF)0$$aGranger, S. J.$$b5
000840068 7001_ $$0P:(DE-HGF)0$$aHernández-Crespo, C.$$b6
000840068 7001_ $$0P:(DE-Juel1)141774$$aHerrmann, F.$$b7
000840068 7001_ $$0P:(DE-HGF)0$$aKeizer, J. J.$$b8
000840068 7001_ $$00000-0001-6875-9978$$aKorkiakoski, M.$$b9
000840068 7001_ $$00000-0001-6058-1466$$aLaudon, H.$$b10
000840068 7001_ $$0P:(DE-HGF)0$$aLehner, I.$$b11
000840068 7001_ $$00000-0001-7892-2708$$aLöfgren, S.$$b12
000840068 7001_ $$00000-0003-3541-672X$$aLohila, A.$$b13
000840068 7001_ $$0P:(DE-HGF)0$$aMacleod, C. J. A.$$b14
000840068 7001_ $$0P:(DE-HGF)0$$aMölder, M.$$b15
000840068 7001_ $$00000-0002-2906-5954$$aMüller, C.$$b16
000840068 7001_ $$0P:(DE-HGF)0$$aNasta, P.$$b17
000840068 7001_ $$0P:(DE-HGF)0$$aNischwitz, V.$$b18
000840068 7001_ $$0P:(DE-HGF)0$$aPaul-Limoges, E.$$b19
000840068 7001_ $$0P:(DE-HGF)0$$aPierret, M. C.$$b20
000840068 7001_ $$00000-0002-5169-5717$$aPilegaard, K.$$b21
000840068 7001_ $$0P:(DE-HGF)0$$aRomano, N.$$b22
000840068 7001_ $$0P:(DE-HGF)0$$aSebastià, M. T.$$b23
000840068 7001_ $$00000-0003-0855-5994$$aStähli, M.$$b24
000840068 7001_ $$0P:(DE-HGF)0$$aVoltz, M.$$b25
000840068 7001_ $$0P:(DE-Juel1)129549$$aVereecken, H.$$b26
000840068 7001_ $$0P:(DE-HGF)0$$aSiemens, J.$$b27
000840068 7001_ $$0P:(DE-Juel1)129484$$aKlumpp, E.$$b28$$eCorresponding author
000840068 773__ $$0PERI:(DE-600)2021601-4$$a10.1002/2017GB005657$$gVol. 31, no. 10, p. 1592 - 1607$$n10$$p1592 - 1607$$tGlobal biogeochemical cycles$$v31$$x0886-6236$$y2017
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