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@ARTICLE{Stroppa:840158,
author = {Stroppa, Daniel G and Righetto, Ricardo D and Montoro,
Luciano A and Houben, Lothar and Barthel, Juri and Cordeiro,
Marco AL and Leite, Edson R and Weng, Weihao and Kiely,
Christopher J and Ramirez, Antonio J},
title = {{A}ssessment of a nanocrystal 3-{D} morphology by the
analysis of single {HAADF}-{HRSTEM} images},
journal = {Nanoscale research letters},
volume = {8},
number = {1},
issn = {1556-276X},
address = {New York, NY [u.a.]},
publisher = {Springer},
reportid = {FZJ-2017-07713},
pages = {475 -},
year = {2013},
abstract = {This work presents the morphological characterization of
CeO2 nanocrystals by the analysis of single unfiltered
high-angle annular dark-field (HAADF)-high-resolution
scanning transmission electron microscopy (HRSTEM) images.
The thickness of each individual atomic column is estimated
by the classification of its HAADF integrated intensity
using a Gaussian mixture model. The resulting thickness maps
obtained from two example nanocrystals with distinct
morphology were analyzed with aid of the symmetry from the
CeO2 crystallographic structure, providing an approximation
for their 3-D morphology with high spatial resolution. A
confidence level of ±1 atom per atomic column along the
viewing direction on the thickness estimation is indicated
by the use of multislice image simulation. The described
characterization procedure stands out as a simple approach
for retrieving morphological parameters of individual
nanocrystals, such as volume and specific surface areas for
different crystalline planes. The procedure is an
alternative to the tilt-series tomography technique for a
number of nanocrystalline systems, since its application
does not require the acquisition of multiple images from the
same nanocrystal along different zone axes},
cin = {ER-C-2},
ddc = {600},
cid = {I:(DE-Juel1)ER-C-2-20170209},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:24225330},
doi = {10.1186/1556-276X-8-475},
url = {https://juser.fz-juelich.de/record/840158},
}