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@ARTICLE{MarcosEsteban:840163,
author = {Marcos Esteban, Raquel and Schütte, Kai and Marquardt,
Dorothea and Barthel, Juri and Beckert, Fabian and
Mülhaupt, Rolf and Janiak, Christoph},
title = {{S}ynthesis of ruthenium@graphene nanomaterials in
propylene carbonate as re-usable catalysts for the
solvent-free hydrogenation of benzene},
journal = {Nano-structures $\&$ nano-objects},
volume = {2},
issn = {2352-507X},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2017-07718},
pages = {28 - 34},
year = {2015},
note = {Dedicated to Prof. Ekkehard Hahn on the occasion of his
60th birthday},
abstract = {Ruthenium nanoparticles (Ru-NPs) can be deposited on
thermally reduced graphite oxide (TRGO) in propylene
carbonate (PC). Propylene carbonate is a biodegradable and
non-toxic solvent. Synthesis of Ru-NPs and deposition on
TRGO were achieved by decomposition of ruthenium
dodecacarbonyl, Ru3(CO)12, by microwave irradiation.
Ru@graphene nanomaterials were identified and characterized
by high resolution transmission electron microscopy (TEM,
HR-TEM), energy-dispersive X-ray diffraction (EDX), selected
area electron diffraction (SAED), X-ray photoelectron
spectroscopy (XPS) and powder X-ray diffraction (PXRD) with
a small diameter and size distribution of Ru-NPs on TRGO.
These Ru@graphene nanomaterials are active catalysts for the
solvent-free hydrogenation of benzene to cyclohexane under
mild conditions (100 °C, 10 bar) with activities of and
over $90\%$ conversion in at least ten consecutive runs.},
cin = {ER-C-2},
ddc = {530},
cid = {I:(DE-Juel1)ER-C-2-20170209},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.nanoso.2015.07.002},
url = {https://juser.fz-juelich.de/record/840163},
}