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| 001 | 840183 | ||
| 005 | 20210129231753.0 | ||
| 024 | 7 | _ | |a 10.1038/am.2017.113 |2 doi |
| 024 | 7 | _ | |a 1884-4049 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2017-07738 |
| 082 | _ | _ | |a 500 |
| 100 | 1 | _ | |a Kleibeuker, Josée E |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Route to achieving perfect B-site ordering in double perovskite thin films |
| 260 | _ | _ | |a Tokyo |c 2017 |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Double perovskites (DP, A2BB’O6) exhibit a breadth of multifunctional properties with a huge potential range of applications, including magneto-optic and spintronic devices. However, spontaneous cation ordering is limited by the similar size and charge of B and B’ cations. We introduce a route to stimulate B-site rock-salt ordering. By growing thin films on (111)-oriented substrates, ‘in-plane’ strain acts on the intrinsically tilted oxygen octahedra of the DP and produces two different B-site cages (in size and shape), stimulating spontaneous cation ordering. For the ferromagnetic insulator La2CoMnO6, clear Co/Mn ordering was achieved by growing on (111)-oriented substrates. The difference in B-site cages was further enhanced when grown under minor (111) in-plane compressive strain, resulting in long-range ordering with a saturation magnetization of 5.8 μB/formula unit (f.u.), close to the theoretical 6 μB/f.u., without antiferromagnetic behavior. Our approach enables the study of many new ordered DPs which have never been made before. |
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| 700 | 1 | _ | |a Choi, Eun-Mi |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Jones, Edward D |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Yu, Tse-Min |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Sala, Bianca |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a MacLaren, Belinda A |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Kepaptsoglou, Demie |0 0000-0003-0499-0470 |b 6 |
| 700 | 1 | _ | |a Hernandez-Maldonado, David |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Ramasse, Quentin M |0 P:(DE-HGF)0 |b 8 |
| 700 | 1 | _ | |a Jones, Lewys |0 0000-0002-6907-0731 |b 9 |
| 700 | 1 | _ | |a Barthel, Juri |0 P:(DE-Juel1)130525 |b 10 |
| 700 | 1 | _ | |a MacLaren, Ian |0 0000-0002-5334-3010 |b 11 |
| 700 | 1 | _ | |a MacManus-Driscoll, Judith L |0 P:(DE-HGF)0 |b 12 |e Corresponding author |
| 773 | _ | _ | |a 10.1038/am.2017.113 |g Vol. 9, no. 7, p. e406 - |0 PERI:(DE-600)2608333-4 |n 7 |p e406 - |t NPG Asia Materials |v 9 |y 2017 |x 1884-4057 |
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