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024 7 _ |a 10.1038/am.2017.113
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100 1 _ |a Kleibeuker, Josée E
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245 _ _ |a Route to achieving perfect B-site ordering in double perovskite thin films
260 _ _ |a Tokyo
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520 _ _ |a Double perovskites (DP, A2BB’O6) exhibit a breadth of multifunctional properties with a huge potential range of applications, including magneto-optic and spintronic devices. However, spontaneous cation ordering is limited by the similar size and charge of B and B’ cations. We introduce a route to stimulate B-site rock-salt ordering. By growing thin films on (111)-oriented substrates, ‘in-plane’ strain acts on the intrinsically tilted oxygen octahedra of the DP and produces two different B-site cages (in size and shape), stimulating spontaneous cation ordering. For the ferromagnetic insulator La2CoMnO6, clear Co/Mn ordering was achieved by growing on (111)-oriented substrates. The difference in B-site cages was further enhanced when grown under minor (111) in-plane compressive strain, resulting in long-range ordering with a saturation magnetization of 5.8 μB/formula unit (f.u.), close to the theoretical 6 μB/f.u., without antiferromagnetic behavior. Our approach enables the study of many new ordered DPs which have never been made before.
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700 1 _ |a Choi, Eun-Mi
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700 1 _ |a Jones, Edward D
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700 1 _ |a Yu, Tse-Min
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700 1 _ |a Sala, Bianca
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700 1 _ |a MacLaren, Belinda A
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700 1 _ |a Kepaptsoglou, Demie
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700 1 _ |a Hernandez-Maldonado, David
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700 1 _ |a Ramasse, Quentin M
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700 1 _ |a Jones, Lewys
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700 1 _ |a Barthel, Juri
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700 1 _ |a MacLaren, Ian
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700 1 _ |a MacManus-Driscoll, Judith L
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773 _ _ |a 10.1038/am.2017.113
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