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@ARTICLE{Kagan:8402,
author = {Kagan, V.E. and Wipf, P. and Stoyanovsky, D. and
Greenberger, J.S. and Borisenko, G. and Belikova, N.A. and
Yanamala, N. and Samhan Arias, A.K. and Tungekar, M.A. and
Jiang, J. and Tyurina, Y.Y. and Ji, J. and
Klein-Seetharaman, J. and Pitt, B.R. and Shvedova, A.A. and
Bayir, H.},
title = {{M}itochondrial targeting of electron scavenging
antioxidants: {R}egulation of selective oxidation vs random
chain reactions},
journal = {Advanced drug delivery reviews},
volume = {61},
issn = {0169-409X},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PreJuSER-8402},
pages = {1375 - 1385},
year = {2009},
note = {This work was supported by NIH Grants U19 AIO68021,
HL70755, HD057587, NS061817, NORA 927Z1LU, PittGrid
(http://www.pittgrid. pitt.edu) and la junta de Extremadura
-Consejeria de Infraestructuras y Desarrollo Tecnologico- y
el Fondo Social Europeo (Orden 2008050288).},
abstract = {Effective regulation of highly compartmentalized production
of reactive oxygen species and peroxidation reactions in
mitochondria requires targeting of small molecule
antioxidants and antioxidant enzymes into the organelles.
This review describes recently developed approaches to
mitochondrial targeting of small biologically active
molecules based on: (i) preferential accumulation in
mitochondria because of their hydrophobicity and positive
charge (hydrophobic cations), (ii) binding with high
affinity to an intra-mitochondrial constituent, and (iii)
metabolic conversions by specific mitochondrial enzymes to
reveal an active entity. In addition, targeted delivery of
antioxidant enzymes via expression of leader sequences
directing the proteins into mitochondria is considered.
Examples of successful antioxidant and anti-apoptotic
protection based on the ability of targeted cargoes to
inhibit cytochrome c-catalyzed peroxidation of a
mitochondria-specific phospholipid cardiolipin, in vitro and
in vivo are presented. Particular emphasis is placed on the
employment of triphenylphosphonium- and hemi-gramicidin
S-moieties as two effective vehicles for mitochondrial
delivery of antioxidants.},
keywords = {Animals / Antioxidants: pharmacology / Apoptosis: drug
effects / Drug Delivery Systems: methods / Electron
Transport Complex I: metabolism / Free Radical Scavengers:
chemistry / Free Radical Scavengers: pharmacokinetics /
Humans / Mitochondria: drug effects / Mitochondria:
metabolism / Models, Biological / Molecular Structure /
Oxidation-Reduction: drug effects / Oxidative Stress: drug
effects / Reactive Oxygen Species: metabolism / Antioxidants
(NLM Chemicals) / Free Radical Scavengers (NLM Chemicals) /
Reactive Oxygen Species (NLM Chemicals) / Electron Transport
Complex I (NLM Chemicals) / J (WoSType)},
cin = {ISB-2},
ddc = {610},
cid = {I:(DE-Juel1)ISB-2-20090406},
pnm = {Programm Biosoft},
pid = {G:(DE-Juel1)FUEK443},
shelfmark = {Pharmacology $\&$ Pharmacy},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:19716396},
pmc = {pmc:PMC2784017},
UT = {WOS:000272600300014},
doi = {10.1016/j.addr.2009.06.008},
url = {https://juser.fz-juelich.de/record/8402},
}