001     840399
005     20210129231828.0
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|a 10.1103/PhysRevX.7.041049
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037 _ _ |a FZJ-2017-07932
082 _ _ |a 530
100 1 _ |0 P:(DE-HGF)0
|a Tymoshenko, Y. V.
|b 0
245 _ _ |a Pseudo-Goldstone Magnons in the Frustrated S=3=2 Heisenberg Helimagnet ZnCr2Se4with a Pyrochlore Magnetic Sublattice
260 _ _ |a College Park, Md.
|b APS
|c 2017
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520 _ _ |a Low-energy spin excitations in any long-range ordered magnetic system in the absence of magnetocrystallineanisotropy are gapless Goldstone modes emanating from the ordering wave vectors. Inhelimagnets, these modes hybridize into the so-called helimagnon excitations. Here we employ neutronspectroscopy supported by theoretical calculations to investigate the magnetic excitation spectrum of theisotropic Heisenberg helimagnet ZnCr2Se4 with a cubic spinel structure, in which spin-3=2 magnetic Cr3þions are arranged in a geometrically frustrated pyrochlore sublattice. Apart from the conventionalGoldstone mode emanating from the ð0 0 qhÞ ordering vector, low-energy magnetic excitations in thesingle-domain proper-screw spiral phase show soft helimagnon modes with a small energy gap of∼0.17 meV, emerging from two orthogonal wave vectors ðqh 00Þ and ð0 qh 0Þ where no magnetic Braggpeaks are present. We term them pseudo-Goldstone magnons, as they appear gapless within linear spinwavetheory and only acquire a finite gap due to higher-order quantum-fluctuation corrections. Our resultsare likely universal for a broad class of symmetric helimagnets, opening up a new way of studying weakmagnon-magnon interactions with accessible spectroscopic methods.
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|a Onykiienko, Y. A.
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|a Müller, T.
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|a Thomale, R.
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|a Rachel, S.
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|a Cameron, A. S.
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|a Portnichenko, P. Y.
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|a Efremov, D. V.
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