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@ARTICLE{Chatterji:840618,
author = {Chatterji, T. and Meven, M. and Brown, P. J.},
title = {{T}emperature evolution of magnetic structure of
{H}o{F}e{O}3 by single crystal neutron diffraction},
journal = {AIP Advances},
volume = {7},
number = {4},
issn = {2158-3226},
address = {New York, NY},
publisher = {American Inst. of Physics},
reportid = {FZJ-2017-08123},
pages = {045106 -},
year = {2017},
abstract = {We have investigated the temperature evolution of the
magnetic structures of HoFeO3 by single crystal neutron
diffraction. The three different magnetic structures
werevfound as a function of temperature for HoFeO3. In all
three phases the fundamental coupling between the Fe
sub-lattices remains the same and only their orientation and
the degree of canting away from the ideal axial direction
varies. The magnetic polarisation of the Ho sub-lattices in
these two higher temperature regions, in which the major
components of the Fe moment lie along x and y, is very
small. The canting of the moments from the axial directions
is attributed to the antisymmetric interactions allowed by
the crystal symmetry. In the low temperature phase two
further structural transitions are apparent in which the
spontaneous magnetisation changes sign with respect to the
underlying antiferromagnetic configuration. In this
temperature range the antisymmetric exchange energy varies
rapidly as the the Ho sub-lattices begin to order. So long
as the ordered Ho moments are small the antisymmetric
exchange is due only to Fe-Fe interactions, but as the
degree of Ho order increases the Fe-Ho interactions take
over whilst at the lowest temperatures, when the Ho moments
approach saturation the Ho-Ho interactions dominate. The
reversals of the spontaneous magnetisation found in this
study suggest that in HoFeO3 the sums of the Fe-Fe and Ho-Ho
antisymmetric interactions have the same sign as one
another, but that of the Ho-Fe terms is opposite.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / JCNS-2},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-2-20110106},
pnm = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)HEIDI-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000400396100027},
doi = {10.1063/1.4979710},
url = {https://juser.fz-juelich.de/record/840618},
}