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@ARTICLE{Tietz:841337,
      author       = {Tietz, Frank},
      title        = {{P}hase relations of {NASICON} materials and compilation of
                      the quaternary phase diagram
                      {N}a$_{2}${O}-{P}$_{2}${O}$_{5}$-{S}i{O}$_{2}$-{Z}r{O}$_{2}$},
      journal      = {AIMS Materials Science},
      volume       = {4},
      number       = {6},
      issn         = {2372-0484},
      address      = {Springfield, Mo.},
      publisher    = {AIMS Press},
      reportid     = {FZJ-2017-08422},
      pages        = {1305 - 1318},
      year         = {2017},
      note         = {open access},
      abstract     = {A short overview is given on existing phase relations in
                      the four related ternary diagrams, setting the frame for a
                      quaternary phase diagram. On the basis of published data the
                      three-dimensional phase region of NASICON materials is
                      constructed and phase relations to ternary and binary
                      systems as well as to single oxides are presented. To date,
                      the NASICON region can be described as a compressed
                      tetrahedron within the tetrahedral phase diagram. However,
                      the three-dimensional presentation clearly elucidates that
                      few reported compositions exist outside this compressed
                      tetrahedron indicating that the phase region of NASICON
                      materials may be larger than the solid solutions known so
                      far. The three-dimensional representation also better
                      elucidates the regions connecting the edges of the NASICON
                      tetrahedron with ternary and binary compounds as well as
                      single oxides, i.e. ZrO2 and ZrSiO4, Na3PO4, sodium
                      silicates and sodium zirconium silicates and gives a better
                      understanding of phase formations during the processing of
                      the ceramics. The implications of the formation of secondary
                      phases and glass-ceramic composites are discussed in terms
                      of technological applications.},
      cin          = {IEK-1 / IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-1-20101013 / I:(DE-Juel1)IEK-12-20141217},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000428531300007},
      doi          = {10.3934/matersci.2017.6.1305},
      url          = {https://juser.fz-juelich.de/record/841337},
}