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@ARTICLE{Broicher:841785,
      author       = {Broicher, Cornelia and Foit, Severin and Rose, Marcus and
                      Hausoul, Peter J. C. and Palkovits, Regina},
      title        = {{A} {B}ipyridine-{B}ased {C}onjugated {M}icroporous
                      {P}olymer for the {I}r-{C}atalyzed {D}ehydrogenation of
                      {F}ormic {A}cid},
      journal      = {ACS catalysis},
      volume       = {7},
      number       = {12},
      issn         = {2155-5435},
      address      = {Washington, DC},
      publisher    = {ACS},
      reportid     = {FZJ-2018-00089},
      pages        = {8413 - 8419},
      year         = {2017},
      abstract     = {Formic acid is considered a promising energy storage
                      medium, and its selective dehydrogenation enables the
                      generation of high-purity H2. Herein we report a
                      bipyridine-based conjugated microporous polymer (CMP) loaded
                      with [Cp*IrCl2]2 for the base-free aqueous dehydrogenation
                      of formic acid to H2/CO2. This catalyst exhibits high
                      activity and selectivity at temperatures over 130 °C and
                      with formic acid concentrations as high as 10 M. Recycling
                      tests demonstrate a low Ir leaching and a gradual increase
                      in the activity over six runs and a low CO content in the
                      gas phase of about 138 ppm. TOFs of up to 123894 h–1 were
                      obtained using 0.1 wt $\%$ Ir loading.},
      cin          = {IEK-9},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-9-20110218},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000417230500047},
      doi          = {10.1021/acscatal.7b02425},
      url          = {https://juser.fz-juelich.de/record/841785},
}