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@ARTICLE{Bonn:842296,
author = {Bonn, Boris and von Schneidemesser, Erika and Butler, Tim
and Churkina, Galina and Ehlers, Christian and Grote,
Rüdiger and Klemp, Dieter and Nothard, Rainer and Schäfer,
Klaus and von Stülpnagel, Albrecht and Kerschbaumer,
Andreas and Yousefpour, Rasoul and Fountoukis, Christos and
Lawrence, Mark G.},
title = {{I}mpact of vegetative emissions on urban ozone and
biogenic secondary organic aerosol: {B}ox model study for
{B}erlin, {G}ermany},
journal = {Journal of cleaner production},
volume = {176},
issn = {0959-6526},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {FZJ-2018-00542},
pages = {827 - 841},
year = {2018},
abstract = {Tropospheric ozone and particulate matter affect human
health and cause vegetation stress, dysfunction and damages.
In this study we investigate the effect of increasing urban
vegetation i.e. tree species on atmospheric chemistry, a
potential urban management strategy to counteract high
levels of local pollutants such as ozone, OH and PM10 caused
by e.g. traffic. We use an extended version of an
atmospheric chemistry box model including detailed gas-phase
chemistry, mixing layer height variation and secondary
organic aerosol calculations based on observations for
Berlin, Germany. It is shown to accurately simulate the
observed ozone volume mixing ratios during the intensive
measurement period in July 2014 (BAERLIN2014) if basic
parameters such as nitrogen oxides, meteorological
conditions, PM10 concentrations as well as volatile organic
compounds (VOCs) are considered as 1 h resolved datasets.
Based on this setup the effects of changing present day
vegetation mixture by 24 different relevant tree species and
of urban greening is tested to elucidate benefits and
drawbacks in order to support future urban planning. While
the present day vegetation causes boundary layer ozone to
decline slightly at 35 °C, individual tree types alter
the ozone production rate and concentration as well as the
secondary organic aerosol mass in different ways. Our
results suggest that trees intensively emitting isoprene
such as black locust, European oak and poplar result in
higher ozone and total PM10 concentrations than at present,
while tree species emitting primarily monoterpenes such as
beech, magnolia and wayfaring trees yield less of both. This
is in line with the similar behaviour of OH concentration
and new particle formation rates. Thus, for future urban
planning including urban greening, consideration of the
beneficial and harmful aspects of tree species need to
ensure that citizens benefit from and are not being
negatively affected by climate adaptation strategies.},
cin = {IEK-8},
ddc = {690},
cid = {I:(DE-Juel1)IEK-8-20101013},
pnm = {243 - Tropospheric trace substances and their
transformation processes (POF3-243)},
pid = {G:(DE-HGF)POF3-243},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000423648000072},
doi = {10.1016/j.jclepro.2017.12.164},
url = {https://juser.fz-juelich.de/record/842296},
}