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@ARTICLE{Erini:842558,
      author       = {Erini, Nina and Beermann, Vera and Gocyla, Martin and
                      Gliech, Manuel and Heggen, Marc and Dunin-Borkowski, Rafal
                      and Strasser, Peter},
      title        = {{T}he {E}ffect of {S}urface {S}ite {E}nsembles on the
                      {A}ctivity and {S}electivity of {E}thanol {E}lectrooxidation
                      by {O}ctahedral {P}t{N}i{R}h {N}anoparticles},
      journal      = {Angewandte Chemie / International edition},
      volume       = {56},
      number       = {23},
      issn         = {1433-7851},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2018-00777},
      pages        = {6533 - 6538},
      year         = {2017},
      abstract     = {Direct ethanol fuel cells are attractive power sources
                      based on a biorenewable, high energy-density fuel. Their
                      efficiency is limited by the lack of active anode materials
                      which catalyze the breaking of the C−C bond coupled to the
                      12-electron oxidation to CO2. We report shape-controlled
                      PtNiRh octahedral ethanol oxidation electrocatalysts with
                      excellent activity and previously unachieved low onset
                      potentials as low as 0.1 V vs. RHE, while being highly
                      selective to complete oxidation to CO2. Our comprehensive
                      characterization and in situ electrochemical ATR studies
                      suggest that the formation of a ternary surface site
                      ensemble around the octahedral Pt3Ni1Rhx nanoparticles plays
                      a crucial mechanistic role for this behavior.},
      cin          = {ER-C-1 / PGI-5},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ER-C-1-20170209 / I:(DE-Juel1)PGI-5-20110106},
      pnm          = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
      pid          = {G:(DE-HGF)POF3-143},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:28455907},
      UT           = {WOS:000401791900030},
      doi          = {10.1002/anie.201702332},
      url          = {https://juser.fz-juelich.de/record/842558},
}