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000842570 1001_ $$00000-0001-5769-0768$$aAviziotis, Ioannis G.$$b0
000842570 245__ $$aChemical Vapor Deposition of Al 13 Fe 4 Highly Selective Catalytic Films for the Semi-Hydrogenation of Acetylene
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000842570 520__ $$aCatalytic properties of coatings containing the Al13Fe4 intermetallic phase are tested in the reaction of semi-hydrogenation of acetylene. The selectivity to ethylene is found as high as 74% close to the reported values for pure, unsupported Al13Fe4. The initial conversion of acetylene to ethylene is 84% and rapidly drops due to the catalytic formation of carbon-based by-products on secondary Al-Fe phases. Coatings are processed through sequential chemical vapor deposition (CVD) of aluminum (5 Torr, 180 °C) and iron (40 Torr, 140 °C) layers, followed by in situ annealing for 60 min at 575 °C. Deposition proceeds at high growth rate, resulting in 15 μm thick films. After annealing, coatings are composed of the Al13Fe4 phase, co-existing with minor secondary Al-Fe intermetallic phases. Overall, it is shown that films containing complex Al-Fe intermetallic phases can be processed by CVD, opening new routes to the engineering of pure, supported Al13Fe4 catalysts on 3D or porous supports.
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000842570 7001_ $$00000-0001-9896-5916$$aDuguet, Thomas$$b1
000842570 7001_ $$0P:(DE-HGF)0$$aSoussi, Khaled$$b2
000842570 7001_ $$0P:(DE-Juel1)130695$$aHeggen, Marc$$b3
000842570 7001_ $$0P:(DE-HGF)0$$aLafont, Marie-Christine$$b4
000842570 7001_ $$0P:(DE-HGF)0$$aMorfin, Franck$$b5
000842570 7001_ $$0P:(DE-HGF)0$$aMishra, Shashank$$b6
000842570 7001_ $$0P:(DE-HGF)0$$aDaniele, Stephane$$b7
000842570 7001_ $$00000-0001-6651-7318$$aBoudouvis, Andreas G.$$b8
000842570 7001_ $$0P:(DE-HGF)0$$aVahlas, Constantin$$b9$$eCorresponding author
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