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@ARTICLE{MacArthur:842613,
author = {MacArthur, Katherine and Brown, Hamish G. and Findlay,
Scott D. and Allen, Leslie J.},
title = {{P}robing the effect of electron channelling on atomic
resolution energy dispersive {X}-ray quantification},
journal = {Ultramicroscopy},
volume = {182},
issn = {0304-3991},
address = {Amsterdam},
publisher = {Elsevier Science},
reportid = {FZJ-2018-00824},
pages = {264 - 275},
year = {2017},
abstract = {Advances in microscope stability, aberration correction and
detector design now make it readily possible to achieve
atomic resolution energy dispersive X-ray mapping for dose
resilient samples. These maps show impressive atomic-scale
qualitative detail as to where the elements reside within a
given sample. Unfortunately, while electron channelling is
exploited to provide atomic resolution data, this very
process makes the images rather more complex to interpret
quantitatively than if no electron channelling occurred.
Here we propose small sample tilt as a means for suppressing
channelling and improving quantification of composition,
whilst maintaining atomic-scale resolution. Only by knowing
composition and thickness of the sample is it possible to
determine the atomic configuration within each column. The
effects of neighbouring atomic columns with differing
composition and of residual channelling on our ability to
extract exact column-by-column composition are also
discussed.},
cin = {ER-C-1},
ddc = {570},
cid = {I:(DE-Juel1)ER-C-1-20170209},
pnm = {143 - Controlling Configuration-Based Phenomena (POF3-143)},
pid = {G:(DE-HGF)POF3-143},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:28780142},
UT = {WOS:000413436500034},
doi = {10.1016/j.ultramic.2017.07.020},
url = {https://juser.fz-juelich.de/record/842613},
}