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024 7 _ |a 10.1103/PhysRevB.97.035404
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100 1 _ |a Messaoudi, Omar
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245 _ _ |a Nondegenerate valleys in the half-metallic ferromagnet Fe / WS 2
260 _ _ |a Woodbury, NY
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520 _ _ |a We present a first-principles investigation of the electronic properties of monolayer WS2 coated with an overlayer of Fe. Our ab initio calculations reveal that the system is a half-metallic ferromagnet with a gap of ∼1 eV for the majority spin channel. Furthermore, the combined effect of time-reversal symmetry breaking due to the magnetic Fe overlayer and the large spin-orbit coupling induced by W gives rise to nondegenerate K and K′ valleys. This has a tremendous impact on the excited-state properties induced by externally applied circularly polarized light. Our analysis demonstrates that the latter induces a singular hot-spot structure of the transition probability around the K and K′ valleys for right and left circular polarization, respectively. We trace back the emergence of this remarkable effect to the strong momentum dependent spin-noncollinearity of the valence band involved. As a main consequence, a strong valley-selective magnetic circular dichroism is obtained, making this system a prime candidate for spintronics and photonics applications.
536 _ _ |a 142 - Controlling Spin-Based Phenomena (POF3-142)
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536 _ _ |a Calculation of quantum spin-fluctuations in nano-magnets (jias19_20161101)
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542 _ _ |i 2018-01-03
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700 1 _ |a Ibañez-Azpiroz, Julen
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700 1 _ |a Bouzar, Hamid
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700 1 _ |a Lounis, Samir
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773 1 8 |a 10.1103/physrevb.97.035404
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773 _ _ |a 10.1103/PhysRevB.97.035404
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