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000843685 1001_ $$0P:(DE-Juel1)164109$$aHackl, Johanna$$b0
000843685 245__ $$aOn the growth mechanisms of polar (100) surfaces of ceria on copper (100)
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000843685 520__ $$aWe present a study of temperature dependent growth of nano-sized ceria islands on a Cu (100) substrate. Low-energy electron microscopy, micro-electron diffraction, X-ray absorption spectroscopy, and photoemission electron microscopy are used to determine the morphology, shape, chemical state, and crystal structure of the grown islands. Utilizing real-time observation capabilities, we reveal a three-way interaction between the ceria, substrate, and local oxygen chemical potential. The interaction manifests in the reorientation of terrace boundaries on the Cu (100) substrate, characteristic of the transition between oxidized and metallic surface. The reorientation is initiated at nucleation sites of ceria islands, whose growth direction is influenced by the proximity of the terrace boundaries. The grown ceria islands were identified as fully stoichiometric CeO2 (100) surfaces with a (2 × 2) reconstruction.
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000843685 7001_ $$0P:(DE-Juel1)165376$$aDuchon, Tomas$$b1$$ufzj
000843685 7001_ $$0P:(DE-HGF)0$$aGottlob, Daniel M.$$b2
000843685 7001_ $$0P:(DE-Juel1)130601$$aCramm, Stefan$$b3
000843685 7001_ $$0P:(DE-HGF)0$$aVeltruská, Kateřina$$b4
000843685 7001_ $$0P:(DE-HGF)0$$aMatolín, Vladimír$$b5
000843685 7001_ $$0P:(DE-Juel1)164137$$aNemšák, Slavomír$$b6$$eCorresponding author
000843685 7001_ $$0P:(DE-Juel1)130948$$aSchneider, Claus M.$$b7
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