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@ARTICLE{Schemme:843726,
author = {Schemme, Steffen and Breuer, Janos and Samsun, Remzi Can
and Peters, Ralf and Stolten, Detlef},
title = {{P}romising catalytic synthesis pathways towards higher
alcohols as suitable transport fuels based on {H}2 and
{CO}2},
journal = {Journal of CO2 utilization},
volume = {27},
issn = {2212-9820},
address = {Amsterdam [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2018-01278},
pages = {223 - 237},
year = {2018},
abstract = {To address the pressing challenges of energy security and
global warming, the coupling of the energy generation and
transport sectors using Power-to-Fuel (PtF) technologies is
an attractive strategy. PtF means the synthesis of transport
fuels based on CO2 from industrial exhaust gases and H2
produced from renewable electricity via electrolysis.This
paper provides a comprehensive overview of the synthesis
possibilities and potentials of H2 and CO2-based methanol
and higher alcohols (C1–C8; from methanol up to octanol)
as alternative transport fuels by adapting established and
novel alcohol synthesis pathways to the PtF concept and
assessing their technical maturity using the Technology
Readiness Level (TRL) method. A literature review reveals
that among the alcohols, methanol, ethanol,
1-/2-/iso-butanol and 1-octanol have the highest relevance
for fuel blending. With the aim to give a first impression,
we roughly estimated and discussed the production costs
depending on the H2 costs. We estimated the TRL of promising
synthesis pathways towards alcohols at 8 for methanol and at
4 for ethanol, 1-butanol and iso-octanol. For 1-octanol, no
suitable synthetic pathway is currently known.},
cin = {IEK-3},
ddc = {624},
cid = {I:(DE-Juel1)IEK-3-20101013},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000445035500024},
doi = {10.1016/j.jcou.2018.07.013},
url = {https://juser.fz-juelich.de/record/843726},
}