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@ARTICLE{Nguyen:843787,
      author       = {Nguyen, Van Nhu and Deja, Robert and Peters, Roland and
                      Blum, Ludger and Stolten, Detlef},
      title        = {{S}tudy of {C}atalytic {C}ombustion of {L}ean
                      {H}ydrogen-{A}ir {M}ixtures in a {M}onolith {R}eactor},
      journal      = {International journal of hydrogen energy},
      volume       = {43},
      number       = {36},
      issn         = {0360-3199},
      address      = {New York, NY [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2018-01330},
      pages        = {17520-17530},
      year         = {2018},
      abstract     = {This paper presents an experimental study of catalytic
                      hydrogen combustion that used commercial catalysts
                      containing Pt in a honeycomb monolith reactor in a plug flow
                      configuration. The emphasis is on determining global
                      kinetics in the case of low hydrogen content. Measurements
                      of the temperature and composition of the reaction product
                      at the outlet in the steady state condition at the different
                      initial compositions of hydrogen and total volumetric feed
                      rates were performed. The conversion of hydrogen was
                      determined in parallel to the composition of the reaction
                      product at the outlet using GC as well as by means of the
                      thermodynamic approach using material and energy balances.
                      The influence of the flow rate and initial molar fraction of
                      hydrogen on hydrogen conversion is shown. A kinetic
                      expression of the Arrhenius type is proposed with the
                      reaction first order in hydrogen and zero order in oxygen
                      for the overall process of the oxidation of hydrogen in lean
                      hydrogen-air mixtures. The determined activation energy was
                      in good agreement with the desorption activation energy for
                      O2 from graphene-covered Pt(111) surfaces using
                      temperature-programmed desorption. This result shows
                      transport-limitations for heterogeneous hydrogen conversion
                      in catalytic hydrogen combustion.},
      cin          = {IEK-3},
      ddc          = {660},
      cid          = {I:(DE-Juel1)IEK-3-20101013},
      pnm          = {135 - Fuel Cells (POF3-135) / SOFC - Solid Oxide Fuel Cell
                      (SOFC-20140602)},
      pid          = {G:(DE-HGF)POF3-135 / G:(DE-Juel1)SOFC-20140602},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000444789300049},
      doi          = {10.1016/j.ijhydene.2018.07.126},
      url          = {https://juser.fz-juelich.de/record/843787},
}