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@ARTICLE{Meier:843822,
      author       = {Meier, G. and Gapinski, J. and Ratajcczyk, M. and Lettinga,
                      M. P. and Hirtz, Kurt and Banachowicz, E. and Patkowski, A.},
      title        = {{N}ano-viscosity of supercooled liquid measured by
                      fluorescence correlation spectroscopy: pressure and
                      temperature dependence and the density scaling},
      journal      = {The journal of chemical physics},
      volume       = {148},
      issn         = {0021-9606},
      address      = {Melville, NY},
      publisher    = {American Institute of Physics},
      reportid     = {FZJ-2018-01361},
      pages        = {094201},
      year         = {2018},
      abstract     = {The Stokes-Einstein relation allows us to calculate
                      apparent viscosity experienced by tracers in complex media
                      on the basis of measured self-diffusion coefficients. Such
                      defined nano-viscosity values can be obtained through single
                      particle techniques, like fluorescence correlation
                      spectroscopy (FCS) and particle tracking (PT). In order to
                      perform such measurements, as functions of pressure and
                      temperature, a new sample cell was designed and is described
                      in this work. We show that this cell in combination with a
                      long working distance objective of the confocal microscope
                      can be used for successful FCS, PT, and confocal imaging
                      experiments in broad pressure (0.1-100 MPa) and temperature
                      ranges. The temperature and pressure dependent
                      nano-viscosity of a van der Waals liquid obtained from the
                      translational diffusion coefficient measured in this cell by
                      means of FCS obeys the same scaling as the rotational
                      relaxation and macro-viscosity of the system.},
      cin          = {ICS-3},
      ddc          = {540},
      cid          = {I:(DE-Juel1)ICS-3-20110106},
      pnm          = {551 - Functional Macromolecules and Complexes (POF3-551)},
      pid          = {G:(DE-HGF)POF3-551},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000427030500017},
      doi          = {10.1063/1.5011196},
      url          = {https://juser.fz-juelich.de/record/843822},
}