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| Hauptseite > Publikationsdatenbank > Nano-viscosity of supercooled liquid measured by fluorescence correlation spectroscopy: pressure and temperature dependence and the density scaling > print |
| Hauptseite > Publikationsdatenbank > Nano-viscosity of supercooled liquid measured by fluorescence correlation spectroscopy: pressure and temperature dependence and the density scaling > print |
| 001 | 843822 | ||
| 005 | 20240619083544.0 | ||
| 024 | 7 | _ | |a 10.1063/1.5011196 |2 doi |
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| 037 | _ | _ | |a FZJ-2018-01361 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |a Meier, G. |0 P:(DE-Juel1)130829 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Nano-viscosity of supercooled liquid measured by fluorescence correlation spectroscopy: pressure and temperature dependence and the density scaling |
| 260 | _ | _ | |a Melville, NY |c 2018 |b American Institute of Physics |
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| 520 | _ | _ | |a The Stokes-Einstein relation allows us to calculate apparent viscosity experienced by tracers in complex media on the basis of measured self-diffusion coefficients. Such defined nano-viscosity values can be obtained through single particle techniques, like fluorescence correlation spectroscopy (FCS) and particle tracking (PT). In order to perform such measurements, as functions of pressure and temperature, a new sample cell was designed and is described in this work. We show that this cell in combination with a long working distance objective of the confocal microscope can be used for successful FCS, PT, and confocal imaging experiments in broad pressure (0.1-100 MPa) and temperature ranges. The temperature and pressure dependent nano-viscosity of a van der Waals liquid obtained from the translational diffusion coefficient measured in this cell by means of FCS obeys the same scaling as the rotational relaxation and macro-viscosity of the system. |
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| 700 | 1 | _ | |a Gapinski, J. |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Ratajcczyk, M. |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Lettinga, M. P. |0 P:(DE-Juel1)130797 |b 3 |
| 700 | 1 | _ | |a Hirtz, Kurt |0 P:(DE-Juel1)130714 |b 4 |
| 700 | 1 | _ | |a Banachowicz, E. |0 P:(DE-HGF)0 |b 5 |
| 700 | 1 | _ | |a Patkowski, A. |0 P:(DE-HGF)0 |b 6 |
| 773 | _ | _ | |a 10.1063/1.5011196 |g Vol. 148, no. 9, p. 094201 - |0 PERI:(DE-600)1473050-9 |p 094201 |t The journal of chemical physics |v 148 |y 2018 |x 0021-9606 |
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