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@ARTICLE{Schwahn:843894,
author = {Schwahn, Dietmar and Pipich, Vitaliy and Kasher, Roni},
title = {{P}hase behavior of methacrylic acid, poly(ethylene glycol)
methyl ether, and poly(ethylene glycol) methacrylate in
aqueous solutions},
journal = {Polymer},
volume = {121},
issn = {0032-3861},
address = {Oxford},
publisher = {Elsevier Science},
reportid = {FZJ-2018-01421},
pages = {111 - 123},
year = {2017},
abstract = {The main issue of this manuscript is the exploration of the
solubility of methacrylic acid (MA), and the oligomers of
poly(ethylene glycol) methyl ether (MPEG), poly(ethylene
glycol) methacrylate (PEGMA), and a mixture of MA and PEGMA.
These solutions obey to the class of associating aqueous
solutions as hydrogen bonding plays an essential role. All
solutions are miscible at ambient temperature. Only a small
fraction of the order of 10−5 molecules is involved in a
process of aggregation forming about 0.4 μm diameter large
colloids whose volume fraction enhances above 70 °C. This
increase of aggregation is going hand and hand with phase
separation of the solution at temperatures at about 70 °C
and above. Spinodal and binodal temperatures of the
solutions were determined from thermal composition
fluctuations following mean field and renormalized 3D-Ising
behavior in dependence of the distance from the spinodal
phase boundary.},
cin = {JCNS (München) ; Jülich Centre for Neutron Science JCNS
(München) ; JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
ddc = {540},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
I:(DE-Juel1)JCNS-1-20110106},
pnm = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6215 / G:(DE-HGF)POF3-6G15 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)KWS1-20140101 / EXP:(DE-MLZ)KWS3-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000405747100013},
doi = {10.1016/j.polymer.2017.06.011},
url = {https://juser.fz-juelich.de/record/843894},
}