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@ARTICLE{Magnani:843906,
      author       = {Magnani, C. and Montis, C. and Mangiapia, G. and Mingotaud,
                      A.-F. and Mingotaud, C. and Roux, C. and Joseph, P. and
                      Berti, D. and Lonetti, B.},
      title        = {{H}ybrid vesicles from lipids and block copolymers: {P}hase
                      behavior from the micro- to the nano-scale},
      journal      = {Colloids and surfaces / B},
      volume       = {168},
      issn         = {0927-7765},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier Science},
      reportid     = {FZJ-2018-01433},
      pages        = {18-28},
      year         = {2018},
      abstract     = {In recent years, there has been a growing interest in the
                      formation of copolymers-lipids hybrid self-assemblies, which
                      allow combining and improving the main features of pure
                      lipids-based and copolymer-based systems known for their
                      potential applications in the biomedical field. In this
                      contribution we investigate the self-assembly behavior of
                      dipalmitoylphosphatidylcholine (DPPC) mixed with
                      poly(butadiene-b-ethyleneoxide) (PBD-PEO), both at the
                      micro- and at the nano-length scale.Epifluorescence
                      microscopy and Laser Scanning Confocal microscopy are
                      employed to characterize the morphology of micron-sized
                      hybrid vesicles. The presence of fluid-like inhomogeneities
                      in their membrane has been evidenced in all the investigated
                      range of compositions. Furthermore, a microfluidic set-up
                      characterizes the mechanical properties of the prepared
                      assemblies by measuring their deformation upon flow: hybrids
                      with low lipid content behave like pure polymer vesicles,
                      whereas objects mainly composed of lipids show more
                      variability from one vesicle to the other. Finally, the
                      structure of the nanosized assemblies is characterized
                      through a combination of Dynamic Light Scattering, Small
                      Angle Neutron Scattering and Transmission Electron
                      Microscopy. A vesicles-to-wormlike transition has been
                      evidenced due to the intimate mixing of DPPC and PBD-PEO at
                      the nanoscale. Combining experimental results at the micron
                      and at the nanoscale improves the fundamental understanding
                      on the phase behavior of copolymer-lipid hybrid assemblies,
                      which is a necessary prerequisite to tailor efficient
                      copolymer-lipid hybrid devices.},
      cin          = {JCNS-FRM-II / Neutronenstreuung ; JCNS-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)JCNS-FRM-II-20110218 /
                      I:(DE-Juel1)JCNS-1-20110106},
      pnm          = {6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
                      Neutron Research (JCNS) (POF3-623)},
      pid          = {G:(DE-HGF)POF3-6G15 / G:(DE-HGF)POF3-6G4},
      experiment   = {EXP:(DE-MLZ)KWS1-20140101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:29395385},
      UT           = {WOS:000443630200004},
      doi          = {10.1016/j.colsurfb.2018.01.042},
      url          = {https://juser.fz-juelich.de/record/843906},
}