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| 100 | 1 | _ | |a Unger, Lana-Simone |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Yttrium doping of Ba 0.5 Sr 0.5 Co 0.8 Fe 0.2 O 3-δ part I: Influence on oxygen permeation, electrical properties, reductive stability, and lattice parameters |
| 260 | _ | _ | |a Amsterdam [u.a.] |c 2018 |b Elsevier Science |
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| 520 | _ | _ | |a Ba0.5Sr0.5Co0.8Fe0.2O3-δ (BSCF) exhibits a very high oxygen permeability in its cubic perovskite phase, making it a promising candidate for high-temperature energy-related applications such as oxygen-transport membranes. It suffers, however, from a pronounced phase instability at application-relevant temperatures below 840 °C which is presumed to result from a valence change of B-site cobalt. In an attempt to stabilize the cubic BSCF phase, monovalent Y3+ was doped in small concentrations (1–10 mol-% yttrium) onto its B-site. The influence of this doping on the physico-chemical properties (electrical conductivity, reductive stability, lattice constant), on the sintering behavior, and on the oxygen permeation of BSCF has been systematically investigated. Despite a slightly adverse effect to permeability (decrease in oxygen permeation by about 20–30%), a doping concentration of 10 mol-% Y is found to completely suppress secondary-phase formation and, hence, stabilize the cubic BSCF system at 800 °C. These findings are extremely promising with regard to a long-term operation of BSCF in atmospheres free of acidic impurity gases. |
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| 700 | 1 | _ | |a Niedrig, Christian |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Wagner, Stefan F. |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Menesklou, Wolfgang |0 P:(DE-HGF)0 |b 3 |
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| 700 | 1 | _ | |a Ivers-Tiffée, Ellen |0 P:(DE-HGF)0 |b 6 |
| 773 | _ | _ | |a 10.1016/j.jeurceramsoc.2017.12.045 |g Vol. 38, no. 5, p. 2378 - 2387 |0 PERI:(DE-600)2013983-4 |n 5 |p 2378 - 2387 |t Journal of the European Ceramic Society |v 38 |y 2018 |x 0955-2219 |
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