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000844525 1001_ $$0P:(DE-HGF)0$$aLi, B.$$b0$$eCorresponding author
000844525 245__ $$aLiquid-like thermal conduction in intercalated layered crystalline solids
000844525 260__ $$aBasingstoke$$bNature Publishing Group$$c2018
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000844525 520__ $$aAs a generic property, all substances transfer heat through microscopic collisions of constituent particles1. A solid conducts heat through both transverse and longitudinal acoustic phonons, but a liquid employs only longitudinal vibrations2,3. As a result, a solid is usually thermally more conductive than a liquid. In canonical viewpoints, such a difference also serves as the dynamic signature distinguishing a solid from a liquid. Here, we report liquid-like thermal conduction observed in the crystalline AgCrSe2. The transverse acoustic phonons are completely suppressed by the ultrafast dynamic disorder while the longitudinal acoustic phonons are strongly scattered but survive, and are thus responsible for the intrinsically ultralow thermal conductivity. This scenario is applicable to a wide variety of layered compounds with heavy intercalants in the van der Waals gaps, manifesting a broad implication on suppressing thermal conduction. These microscopic insights might reshape the fundamental understanding on thermal transport properties of matter and open up a general opportunity to optimize performances of thermoelectrics.
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000844525 7001_ $$00000-0001-9972-2019$$aWang, H.$$b1
000844525 7001_ $$0P:(DE-HGF)0$$aKawakita, Y.$$b2
000844525 7001_ $$00000-0003-0389-7039$$aZhang, Q.$$b3
000844525 7001_ $$0P:(DE-Juel1)169262$$aFeygenson, M.$$b4$$ufzj
000844525 7001_ $$0P:(DE-HGF)0$$aYu, H. L.$$b5
000844525 7001_ $$0P:(DE-HGF)0$$aWu, D.$$b6
000844525 7001_ $$0P:(DE-HGF)0$$aOhara, K.$$b7
000844525 7001_ $$0P:(DE-HGF)0$$aKikuchi, T.$$b8
000844525 7001_ $$0P:(DE-HGF)0$$aShibata, K.$$b9
000844525 7001_ $$0P:(DE-HGF)0$$aYamada, T.$$b10
000844525 7001_ $$0P:(DE-HGF)0$$aNing, X. K.$$b11
000844525 7001_ $$0P:(DE-HGF)0$$aChen, Y.$$b12
000844525 7001_ $$0P:(DE-HGF)0$$aHe, J. Q.$$b13
000844525 7001_ $$0P:(DE-HGF)0$$aVaknin, D.$$b14
000844525 7001_ $$0P:(DE-HGF)0$$aWu, R. Q.$$b15
000844525 7001_ $$0P:(DE-HGF)0$$aNakajima, K.$$b16
000844525 7001_ $$0P:(DE-HGF)0$$aKanatzidis, M. G.$$b17
000844525 773__ $$0PERI:(DE-600)2088679-2$$a10.1038/s41563-017-0004-2$$gVol. 17, no. 3, p. 226 - 230$$n3$$p226 - 230$$tNature materials$$v17$$x1476-4660$$y2018
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