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@ARTICLE{Li:844525,
author = {Li, B. and Wang, H. and Kawakita, Y. and Zhang, Q. and
Feygenson, M. and Yu, H. L. and Wu, D. and Ohara, K. and
Kikuchi, T. and Shibata, K. and Yamada, T. and Ning, X. K.
and Chen, Y. and He, J. Q. and Vaknin, D. and Wu, R. Q. and
Nakajima, K. and Kanatzidis, M. G.},
title = {{L}iquid-like thermal conduction in intercalated layered
crystalline solids},
journal = {Nature materials},
volume = {17},
number = {3},
issn = {1476-4660},
address = {Basingstoke},
publisher = {Nature Publishing Group},
reportid = {FZJ-2018-01935},
pages = {226 - 230},
year = {2018},
abstract = {As a generic property, all substances transfer heat through
microscopic collisions of constituent particles1. A solid
conducts heat through both transverse and longitudinal
acoustic phonons, but a liquid employs only longitudinal
vibrations2,3. As a result, a solid is usually thermally
more conductive than a liquid. In canonical viewpoints, such
a difference also serves as the dynamic signature
distinguishing a solid from a liquid. Here, we report
liquid-like thermal conduction observed in the crystalline
AgCrSe2. The transverse acoustic phonons are completely
suppressed by the ultrafast dynamic disorder while the
longitudinal acoustic phonons are strongly scattered but
survive, and are thus responsible for the intrinsically
ultralow thermal conductivity. This scenario is applicable
to a wide variety of layered compounds with heavy
intercalants in the van der Waals gaps, manifesting a broad
implication on suppressing thermal conduction. These
microscopic insights might reshape the fundamental
understanding on thermal transport properties of matter and
open up a general opportunity to optimize performances of
thermoelectrics.},
cin = {ICS-1 / Neutronenstreuung ; JCNS-1 / JCNS-ESS},
ddc = {610},
cid = {I:(DE-Juel1)ICS-1-20110106 / I:(DE-Juel1)JCNS-1-20110106 /
I:(DE-Juel1)JCNS-ESS-20170404},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551) /
6G4 - Jülich Centre for Neutron Research (JCNS) (POF3-623)
/ 6215 - Soft Matter, Health and Life Sciences (POF3-621)},
pid = {G:(DE-HGF)POF3-551 / G:(DE-HGF)POF3-6G4 /
G:(DE-HGF)POF3-6215},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:29335610},
UT = {WOS:000426012000010},
doi = {10.1038/s41563-017-0004-2},
url = {https://juser.fz-juelich.de/record/844525},
}