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@ARTICLE{Pipich:844610,
author = {Pipich, Vitaliy and Schwahn, Dietmar},
title = {{D}ensification of {S}upercritical {C}arbon {D}ioxide
{A}ccompanied by {D}roplet {F}ormation {W}hen {P}assing the
{W}idom {L}ine},
journal = {Physical review letters},
volume = {120},
number = {14},
issn = {0031-9007},
address = {College Park, Md.},
publisher = {APS},
reportid = {FZJ-2018-02012},
pages = {145701},
year = {2018},
abstract = {Thermal density fluctuations of supercritical CO2 were
explored using small-angle neutron scattering (SANS), whose
amplitude (susceptibility) and correlation length show the
expected maximum at the Widom line. At low pressure, the
susceptibility is in excellent agreement with the evaluated
values on the basis of mass density measurements. At about
20 bar beyond the Widom line, SANS shows the formation of
droplets accompanied by an enhanced number density of the
supercritical fluid. The corresponding borderline is
interpreted as a Frenkel line separating gas- and liquidlike
regimes.},
cin = {Neutronenstreuung ; JCNS-1 / JCNS (München) ; Jülich
Centre for Neutron Science JCNS (München) ; JCNS-FRM-II},
ddc = {550},
cid = {I:(DE-Juel1)JCNS-1-20110106 /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
6G15 - FRM II / MLZ (POF3-6G15) / 6G4 - Jülich Centre for
Neutron Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-6215 / G:(DE-HGF)POF3-6G15 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)KWS1-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000429227100005},
doi = {10.1103/PhysRevLett.120.145701},
url = {https://juser.fz-juelich.de/record/844610},
}