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000844653 1001_ $$0P:(DE-Juel1)156533$$aEsat, Taner$$b0$$ufzj
000844653 245__ $$aA standing molecule as a single-electron field emitter
000844653 260__ $$aLondon [u.a.]$$bNature Publ. Group$$c2018
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000844653 520__ $$aScanning probe microscopy makes it possible to image and spectroscopically characterize nanoscale objects, and to manipulate1,2,3 and excite4,5,6,7,8 them; even time-resolved experiments are now routinely achieved9,10. This combination of capabilities has enabled proof-of-principle demonstrations of nanoscale devices, including logic operations based on molecular cascades11, a single-atom transistor12, a single-atom magnetic memory cell13 and a kilobyte atomic memory14. However, a key challenge is fabricating device structures that can overcome their attraction to the underlying surface and thus protrude from the two-dimensional flatlands of the surface. Here we demonstrate the fabrication of such a structure: we use the tip of a scanning probe microscope to lift a large planar aromatic molecule (3,4,9,10-perylenetetracarboxylic-dianhydride) into an upright, standing geometry on a pedestal of two metal (silver) adatoms. This atypical and surprisingly stable upright orientation of the single molecule, which under all known circumstances adsorbs flat on metals15,16, enables the system to function as a coherent single-electron field emitter. We anticipate that other metastable adsorbate configurations might also be accessible, thereby opening up the third dimension for the design of functional nanostructures on surfaces.
000844653 536__ $$0G:(DE-HGF)POF3-142$$a142 - Controlling Spin-Based Phenomena (POF3-142)$$cPOF3-142$$fPOF III$$x0
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000844653 7001_ $$0P:(DE-Juel1)171486$$aFriedrich, Niklas$$b1
000844653 7001_ $$0P:(DE-Juel1)128791$$aTautz, F. Stefan$$b2$$eCorresponding author$$ufzj
000844653 7001_ $$0P:(DE-Juel1)128792$$aTemirov, Ruslan$$b3$$ufzj
000844653 773__ $$0PERI:(DE-600)1413423-8$$a10.1038/s41586-018-0223-y$$gVol. 558, no. 7711, p. 573 - 576$$n7711$$p573 - 576$$tNature <London>$$v558$$x0028-0836$$y2018
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