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@ARTICLE{Tang:844896,
author = {Tang, H. and Kochetkova, T. and Kriegs, H. and Dhont, Jan
K.G. and Lettinga, M. P.},
title = {{S}hear-banding in entangled xanthan solutions: tunable
transition from sharp to broad shear-band interfaces},
journal = {Soft matter},
volume = {14},
number = {5},
issn = {1744-6848},
address = {London},
publisher = {Royal Soc. of Chemistry},
reportid = {FZJ-2018-02238},
pages = {826 - 836},
year = {2018},
abstract = {We report on the smooth transition between gradient-banded
velocity profiles with a sharp interface and curved velocity
profiles, both resulting from strong shear-thinning
dispersions of concentrated xanthan (a highly charged
poly-saccharide). Pronounced shear-banded flow, where two
extended shear-bands are separated by a relatively sharp
interface, is observed in a limited range of shear rates, at
very low ionic strength and at a high concentration, using
heterodyne light scattering to measure spatially resolved
velocity profiles. The width of the interface between the
coexisting shear-bands broadens to span a sizable fraction
of the gap of the shear cell, either by changing the shear
rate, by lowering the concentration, or by increasing the
ionic strength. The broadening results in a smooth
transition to highly curved velocity profiles and is
connected to a disappearing flow birefringence. Thus, these
experiments show that the classic shear-banding instability
can give rise to highly curved velocity profiles, due to the
existence of broad interfaces between the bands, with an
extent of the order or larger than the cell gap width. This
observation may aid to resolve the ongoing dispute
concerning shear-banding of highly entangled polymeric
systems, suggesting that the curved velocity profiles that
have been observed in the past are in fact shear-banded
states with an unusually broad interface.},
cin = {ICS-3},
ddc = {530},
cid = {I:(DE-Juel1)ICS-3-20110106},
pnm = {551 - Functional Macromolecules and Complexes (POF3-551)},
pid = {G:(DE-HGF)POF3-551},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:29308827},
UT = {WOS:000423996300017},
doi = {10.1039/C7SM01734K},
url = {https://juser.fz-juelich.de/record/844896},
}