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000844897 1001_ $$0P:(DE-HGF)0$$aRuiz-Franco, J.$$b0
000844897 245__ $$aCrystal-to-Crystal Transition of Ultrasoft Colloids under Shear
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000844897 520__ $$aUltrasoft colloids typically do not spontaneously crystallize, but rather vitrify, at high concentrations. Combining in situ rheo–small-angle-neutron-scattering experiments and numerical simulations we show that shear facilitates crystallization of colloidal star polymers in the vicinity of their glass transition. With increasing shear rate well beyond rheological yielding, a transition is found from an initial bcc-dominated structure to an fcc-dominated one. This crystal-to-crystal transition is not accompanied by intermediate melting but occurs via a sudden reorganization of the crystal structure. Our results provide a new avenue to tailor colloidal crystallization and the crystal-to-crystal transition at the molecular level by coupling softness and shear.
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000844897 7001_ $$0P:(DE-HGF)0$$aMarakis, J.$$b1
000844897 7001_ $$0P:(DE-HGF)0$$aGnan, N.$$b2
000844897 7001_ $$0P:(DE-HGF)0$$aKohlbrecher, J.$$b3
000844897 7001_ $$0P:(DE-HGF)0$$aGauthier, M.$$b4
000844897 7001_ $$0P:(DE-Juel1)130797$$aLettinga, M.P.$$b5$$ufzj
000844897 7001_ $$0P:(DE-HGF)0$$aVlassopoulos, D.$$b6$$eCorresponding author
000844897 7001_ $$0P:(DE-HGF)0$$aZaccarelli, E.$$b7$$eCorresponding author
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