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100 1 _ |a Ruiz-Franco, J.
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245 _ _ |a Crystal-to-Crystal Transition of Ultrasoft Colloids under Shear
260 _ _ |a College Park, Md.
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520 _ _ |a Ultrasoft colloids typically do not spontaneously crystallize, but rather vitrify, at high concentrations. Combining in situ rheo–small-angle-neutron-scattering experiments and numerical simulations we show that shear facilitates crystallization of colloidal star polymers in the vicinity of their glass transition. With increasing shear rate well beyond rheological yielding, a transition is found from an initial bcc-dominated structure to an fcc-dominated one. This crystal-to-crystal transition is not accompanied by intermediate melting but occurs via a sudden reorganization of the crystal structure. Our results provide a new avenue to tailor colloidal crystallization and the crystal-to-crystal transition at the molecular level by coupling softness and shear.
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700 1 _ |a Marakis, J.
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700 1 _ |a Gnan, N.
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700 1 _ |a Kohlbrecher, J.
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700 1 _ |a Gauthier, M.
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700 1 _ |a Vlassopoulos, D.
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700 1 _ |a Zaccarelli, E.
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773 _ _ |a 10.1103/PhysRevLett.120.078003
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