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@ARTICLE{Rupp:845041,
author = {Rupp, Jonathan A. J. and Querré, Madec and Kindsmüller,
Andreas and Besland, Marie-Paule and Janod, Etienne and
Dittmann, Regina and Waser, R. and Wouters, Dirk J.},
title = {{D}ifferent threshold and bipolar resistive switching
mechanisms in reactively sputtered amorphous undoped and
{C}r-doped vanadium oxide thin films},
journal = {Journal of applied physics},
volume = {123},
number = {4},
issn = {1089-7550},
address = {Melville, NY},
publisher = {American Inst. of Physics},
reportid = {FZJ-2018-02370},
pages = {044502 -},
year = {2018},
abstract = {This study investigates resistive switching in amorphous
undoped and Cr-doped vanadium oxide thin films synthesized
by sputtering deposition at low oxygen partial pressure. Two
different volatile threshold switching characteristics can
occur as well as a non-volatile bipolar switching mechanism,
depending on device stack symmetry and Cr-doping. The two
threshold switching types are associated with different
crystalline phases in the conduction filament created during
an initial forming step. The first kind of threshold
switching, observed for undoped vanadium oxide films, was,
by its temperature dependence, proven to be associated with
a thermally triggered insulator-to-metal transition in a
crystalline VO2 phase, whereas the threshold switch observed
in chromium doped films is stable up to 90 °C and shows
characteristics of an electronically induced Mott
transition. This different behaviour for undoped versus
doped films has been attributed to an increased stability of
V3+ due to the Cr3+ doping (as evidenced by X-ray
photoelectron spectroscopy analysis), probably favouring the
creation of a crystalline Cr-doped V2O3 phase (rather than a
Cr-doped VO2 phase) during the energetic forming step. The
symmetric Pt/a-(VCr)Ox/Pt device showing high temperature
stable threshold switching may find interesting applications
as a possible new selector device for resistive switching
memory (ReRAM) crossbar arrays.I. INTRODUCTION},
cin = {PGI-7 / JARA-FIT},
ddc = {530},
cid = {I:(DE-Juel1)PGI-7-20110106 / $I:(DE-82)080009_20140620$},
pnm = {521 - Controlling Electron Charge-Based Phenomena
(POF3-521)},
pid = {G:(DE-HGF)POF3-521},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000423875800035},
doi = {10.1063/1.5006145},
url = {https://juser.fz-juelich.de/record/845041},
}