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@ARTICLE{Scheepers:845361,
author = {Scheepers, Fabian and Burdzik, Andrea and Stähler, Markus
and Carmo, Marcelo and Lehnert, Werner and Stolten, Detlef},
title = {{A} {N}ew {S}etup for the {Q}uantitive {A}nalysis of
{D}rying by the {U}se of {G}as-phase {FTIR}-{S}pectroscopy},
journal = {Review of scientific instruments},
volume = {89},
number = {8},
issn = {0034-6748},
address = {[S.l.]},
publisher = {American Institute of Physics},
reportid = {FZJ-2018-02635},
pages = {083102 -},
year = {2018},
abstract = {Drying rates are important for the manufacture of thin
films and in specific for the production of electrodes used
in electrochemical devices such as fuel cells and
electrolyzers. The known procedures to investigate
time-dependent sample compositions and selective evaporation
rates are insufficient to obtain mean information about the
full area instead of a single point analysis. Therefore, a
new setup is presented using gas-phase Fourier-transform
infrared spectroscopy. This method analyzes the gas-phase
composition to recalculate the layer composition in
electrode fabrication at any time during drying. According
to the golden rule of measurement technology, manufacturer
specifications are often overestimated. Therefore, our
alternative procedures were used to evaluate the precision
of devices used. The calculated measurement precision is
confirmed by validation. The expected deviation is
quantified to be less than $2\%$ for the common application.
Further on, the relative test-retest standard deviation is
determined to be $0.3\%–0.4\%.$ As a result of the error
propagation, the measurement precision is limited by the
background gas flow rate precision for common application.
At low volume fractions, the influence of the substance flow
rate deviations becomes significant. However, further
studies will focus on increasing the gas flow rate
precision},
cin = {IEK-3},
ddc = {530},
cid = {I:(DE-Juel1)IEK-3-20101013},
pnm = {135 - Fuel Cells (POF3-135)},
pid = {G:(DE-HGF)POF3-135},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:30184627},
UT = {WOS:000443720400003},
doi = {10.1063/1.5036817},
url = {https://juser.fz-juelich.de/record/845361},
}