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@ARTICLE{Ferraresi:845415,
      author       = {Ferraresi, Giulio and El Kazzi, Mario and Czornomaz, Lukas
                      and Tsai, Chih-Long and Uhlenbruck, Sven and Villevieille,
                      Claire},
      title        = {{E}lectrochemical {P}erformance of {A}ll-{S}olid-{S}tate
                      {L}i-{I}on {B}atteries {B}ased on {G}arnet {E}lectrolyte
                      {U}sing {S}ilicon as a {M}odel {E}lectrode},
      journal      = {ACS energy letters},
      volume       = {3},
      number       = {4},
      issn         = {2380-8195},
      address      = {Washington, DC},
      publisher    = {American Chemical Society},
      reportid     = {FZJ-2018-02683},
      pages        = {1006 - 1012},
      year         = {2018},
      abstract     = {Owing to improved safety, all-solid-state batteries based
                      on the garnet Ta-substituted Li7La3Zr2O12 solid electrolyte
                      are promising alternatives to conventional Li-ion batteries
                      with organic electrolytes. However, to date, the viability
                      of such all-solid-state batteries is uncertain because their
                      performance is limited by the problematic
                      electrode−electrolyte interface. Herein, we report the
                      viability to use Si anodes facilitated by enhancement of
                      this interface. Before depositing Si as a thin film
                      electrode (50 nm) on the smooth surface of the solid
                      electrolyte, we treated the electrolyte surface by argon
                      plasma etching to reduce the amount of resistive species.
                      This approach enabled the cycling of Si/garnet/Li
                      all-solid-state cells, achieving an initial capacity of
                      ~2700 mAh/g followed by partial fading and stabilization for
                      more than 100 cycles. Electrochemical measurement, coupled
                      with morphological and chemical investigations, demonstrate
                      that Si is a viable anode in combination with garnet
                      electrolyte and emphasize the importance of controlling the
                      solid/solid interface.},
      cin          = {IEK-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {131 - Electrochemical Storage (POF3-131)},
      pid          = {G:(DE-HGF)POF3-131},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000430369600034},
      doi          = {10.1021/acsenergylett.8b00264},
      url          = {https://juser.fz-juelich.de/record/845415},
}