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@ARTICLE{Reim:845494,
author = {Reim, Johannes and Rosén, E. and Zaharko, O. and Mostovoy,
M. and Robert, J. and Valldor, M. and Schweika, W.},
title = {{N}eutron diffraction study and theoretical analysis of the
antiferromagnetic order and the diffuse scattering in the
layered kagome system {C}a{B}a{C}o$_2${F}e$_2${O}$_7$},
journal = {Physical review / B},
volume = {97},
number = {14},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {FZJ-2018-02728},
pages = {144402},
year = {2018},
abstract = {The hexagonal swedenborgite, CaBaCo2Fe2O7, is a chiral
frustrated antiferromagnet, in which magnetic ions form
alternating kagome and triangular layers. We observe a
long-range √3×√3 antiferromagnetic order setting in
below TN=160 K by neutron diffraction on single crystals of
CaBaCo2Fe2O7. Both magnetization and polarized neutron
single crystal diffraction measurements show that close to
TN spins lie predominantly in the ab plane, while upon
cooling the spin structure becomes increasingly canted due
to Dzyaloshinskii-Moriya interactions. The ordered structure
can be described and refined within the magnetic space group
P31m′. Diffuse scattering between the magnetic peaks
reveals that the spin order is partial. Monte Carlo
simulations based on a Heisenberg model with two
nearest-neighbor exchange interactions show a similar
diffuse scattering and coexistence of the √3×√3 order
with disorder. The coexistence can be explained by the
freedom to vary spins without affecting the long-range
order, which gives rise to ground-state degeneracy.
Polarization analysis of the magnetic peaks indicates the
presence of long-period cycloidal spin correlations
resulting from the broken inversion symmetry of the lattice,
in agreement with our symmetry analysis.},
cin = {JCNS-2 / PGI-4 / JARA-FIT / JCNS-FRM-II},
ddc = {530},
cid = {I:(DE-Juel1)JCNS-2-20110106 / I:(DE-Juel1)PGI-4-20110106 /
$I:(DE-82)080009_20140620$ /
I:(DE-Juel1)JCNS-FRM-II-20110218},
pnm = {144 - Controlling Collective States (POF3-144) / 524 -
Controlling Collective States (POF3-524) / 6212 - Quantum
Condensed Matter: Magnetism, Superconductivity (POF3-621) /
6213 - Materials and Processes for Energy and Transport
Technologies (POF3-621) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (POF3-623)},
pid = {G:(DE-HGF)POF3-144 / G:(DE-HGF)POF3-524 /
G:(DE-HGF)POF3-6212 / G:(DE-HGF)POF3-6213 /
G:(DE-HGF)POF3-6G4},
experiment = {EXP:(DE-MLZ)DNS-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000429208800006},
doi = {10.1103/PhysRevB.97.144402},
url = {https://juser.fz-juelich.de/record/845494},
}